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Volz, Jessica B; Geibert, Walter; Koehler, Dennis; Rutgers van der Loeff, Michiel M; Kasten, Sabine (2022): Distribution of radioisotopes in polymetallic nodules from the CCZ collected during SONNE cruise SO239 [dataset]. PANGAEA, https://doi.org/10.1594/PANGAEA.951145

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Published: 2022-11-21DOI registered: 2023-01-03

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Abstract:
This dataset comprises gamma spectrometric measurements of radioisotopes in samples from polymetallic nodules, which were collected in the framework of the European collaborative JPI Oceans MiningImpact project onboard R/V SONNE cruise SO239 in 2015. Samples were taken from different parts of the nodules (topside surface (s), bottom surface (b), interior (i)). The gamma radiation was measured in a Canberra well-type HPGe detector. Emission lines at 46 keV (Pb-210), 63 keV (U-234 via Th-234), 67 keV (Th-230), 186 keV (Ra-226 in absence of U-235 interference), 295 keV (Ra-226 via Rn-222) and 402 keV (Pa-231 via Rn-219 with some uncertainty on the intermediate Pa-231/Ac-227 equilibrium) were evaluated. The diluted uranium ore standard RGU-1 and the uranium ore standard UREM-11 served as calibration and reference, respectively.
Keyword(s):
Clarion Clipperton Fracture Zone; isotope data; polymetallic nodules; Radioactivity
Supplement to:
Volz, Jessica B; Geibert, Walter; Koehler, Dennis; Rutgers van der Loeff, Michiel M; Kasten, Sabine (2023): Alpha radiation from polymetallic nodules and potential health risks from deep-sea mining. Scientific Reports, 13(1), 7985, https://doi.org/10.1038/s41598-023-33971-w
Project(s):
Funding:
Federal Ministry of Education and Research (BMBF), grant/award no. 03F0812F: JPI-O MiningImpact: Auswirkungen von Manganknollenbergbau auf biogeochemische Prozesse und die Ausbreitung von Stoffen in der Tiefsee
Coverage:
Median Latitude: 13.916668 * Median Longitude: -123.792066 * South-bound Latitude: 11.079000 * West-bound Longitude: -130.136330 * North-bound Latitude: 18.795830 * East-bound Longitude: -117.550330
Date/Time Start: 2015-03-29T04:18:00 * Date/Time End: 2015-04-21T20:08:00
Minimum Elevation: -4936.4 m * Maximum Elevation: -4324.5 m
Event(s):
SO239_60-1 (BC9) * Latitude: 11.807670 * Longitude: -117.550330 * Date/Time: 2015-03-29T04:18:00 * Elevation: -4324.5 m * Location: North Pacific Ocean * Campaign: SO239 * Basis: Sonne_2 * Method/Device: Box corer (BC) * Comment: German BGR
SO239_88-1 * Latitude: 11.079000 * Longitude: -119.658830 * Date/Time: 2015-04-02T19:42:00 * Elevation: -4432.9 m * Location: North Pacific Ocean * Campaign: SO239 * Basis: Sonne_2 * Method/Device: Box corer (BC) * Comment: IOM Joint Org.
SO239_119-1 (BC20) * Latitude: 13.859170 * Longitude: -123.252670 * Date/Time: 2015-04-08T08:06:00 * Elevation: -4516.2 m * Location: North Pacific Ocean * Campaign: SO239 * Basis: Sonne_2 * Method/Device: Box corer (BC) * Comment: Belgian GSR
Comment:
RGU-1 (400 ppm U) was used for calibration. Except for U (186 keV!), activities are very similar to nodules.
Parameter(s):
#NameShort NameUnitPrincipal InvestigatorMethod/DeviceComment
1Event labelEventVolz, Jessica B
2Sample code/labelSample labelVolz, Jessica B
3Depth, top/minDepth topmVolz, Jessica B
4Depth, bottom/maxDepth botmVolz, Jessica B
5Sample typeSamp typeVolz, Jessica Bnodule
6Sample massSamp mgVolz, Jessica B
7Time in secondsTime secsVolz, Jessica BCounting time
8Lead-210210Pbdpm/gVolz, Jessica B46 keV
9Lead-210, error210Pb e±Volz, Jessica B1 s error (only counting, absolute units)
10Uranium-234234Udpm/gVolz, Jessica Bvia 234Th (63 keV)
11Uranium-234, error234U e±Volz, Jessica B1 s error (only counting, absolute units)
12Thorium-230230Thdpm/gVolz, Jessica B67 keV; Unfortunate, probably random peak deconvolution for 230Th (see measured vs. expected value for UREM-11)
13Thorium-230, error230Th e±Volz, Jessica B1 s error (only counting, absolute units)
14Radium-226226Radpm/gVolz, Jessica B186 keV; For RGU-1 and UREM-11, this gamma line has a 235U interference (see measured vs. expected value for UREM-11) but not for the nodules. Good correlation of 226Ra (direct) vs. 226Ra (via 222Rn) for nodules, but precision is only 70%
15Radium-226, error226Ra e±Volz, Jessica B1 s error (only counting, absolute units)
16Radium-226226Radpm/gVolz, Jessica Bvia 222Rn (295 keV); Best value for 226Ra
17Radium-226, error226Ra e±Volz, Jessica B1 s error (only counting, absolute units)
18Radon-222222Rndpm/gVolz, Jessica B351 keV; values with #: 2 peaks manually added
19Radon-222, error222Rn e±Volz, Jessica B1 s error (only counting, absolute units)
20Protactinium-231231Padpm/gVolz, Jessica B227Ac, 219Rn 6.7% (402 keV); Gamma line for 231Pa chosen based on Geibert, W. (2001): Actinium-227 als Tracer für Advektion und Mischung in der Tiefsee , PhD thesis, Universität Bremen. Some uncertainty on the intermediate 231Pa/227Ac equilibrium
21Protactinium-231, error231Pa e±Volz, Jessica B1 s error (only counting, absolute units)
22Radon-222222Rndpm/gVolz, Jessica B609 keV
23Radon-222, error222Rn e±Volz, Jessica B1 s error (only counting, absolute units)
Status:
Curation Level: Enhanced curation (CurationLevelC)
Size:
440 data points

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