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Asmala, Eero; Haraguchi, Lumi; Markager, Stiig; Massicotte, Philippe; Riemann, Bo; Staehr, Peter A; Carstensen, Jacob (2018): Water column nutrient, chlorophyll and dissolved organic carbon concentrations and dissolved organic matter characteristics in Roskilde Fjord, Denmark [dataset]. PANGAEA, https://doi.org/10.1594/PANGAEA.895734, Supplement to: Asmala, E et al. (2018): Eutrophication leads to accumulation of recalcitrant autochthonous organic matter in coastal environment. Global Biogeochemical Cycles, 32(11), 1673-1687, https://doi.org/10.1029/2017GB005848

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Published: 2018-11-02DOI registered: 2019-02-23

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Abstract:
Anthropogenic nutrient enrichment is changing the structure and the function of coastal ecosystems. These coastal zones are transitions between freshwater and marine systems where multiple biogeochemical processes remove, produce and transform organic matter. The extent to which the coastal zone is merely a conduit for terrestrial (allochthonous) organic matter, versus a distinct source of autochthonous organic matter fueled by eutrophication, is unclear. To address this issue, we characterized the freshwater and marine dissolved organic matter (DOM) pools in an eutrophic estuary with a long water residence time (Roskilde Fjord, Denmark) over an annual cycle. We combined elemental, optical (absorbance and fluorescence) and isotopic analyses to obtain insight about the bulk properties of the DOM pool during this period. We also used sediment traps to analyze the changes related to the exchange of organic matter between the particulate (POM) and dissolved (DOM) fractions. The results showed that labile autochthonous DOM from in situ primary production was rapidly transformed to more recalcitrant DOM that accumulated in the estuary despite continuous exchange with the open sea. Also, parts of the POM pool were degraded rapidly (within 24h) and transformed into the DOM pool. Accumulated DOM was characterized by relatively low molecular size and stable carbon isotopic value, and by high protein-like fluorescence. These results indicate that autotrophic material can be a major source of specific recalcitrant DOM in eutrophic coastal waters, contributing significantly to the flux of organic carbon to the ocean.
Coverage:
Median Latitude: 55.813383 * Median Longitude: 12.019381 * South-bound Latitude: 55.650000 * West-bound Longitude: 11.887220 * North-bound Latitude: 55.937220 * East-bound Longitude: 12.120560
Date/Time Start: 2014-04-28T00:00:00 * Date/Time End: 2015-11-25T00:00:00
Minimum DEPTH, water: m * Maximum DEPTH, water: m
Event(s):
Roskilde_fjord_RF01 * Latitude: 55.713330 * Longitude: 12.066670 * Method/Device: Multiple investigations (MULT) * Comment: Sampled from shore
Roskilde_fjord_RF02 * Latitude: 55.922780 * Longitude: 12.020600 * Method/Device: Multiple investigations (MULT) * Comment: Sampled from shore
Roskilde_fjord_RF03 * Latitude: 55.937220 * Longitude: 11.887220 * Method/Device: Multiple investigations (MULT) * Comment: Sampled from shore
Parameter(s):
#NameShort NameUnitPrincipal InvestigatorMethod/DeviceComment
1Event labelEventAsmala, Eero
2Sample IDSample IDAsmala, Eero
3DATE/TIMEDate/TimeAsmala, EeroGeocode
4LATITUDELatitudeAsmala, EeroGeocode
5LONGITUDELongitudeAsmala, EeroGeocode
6Nitrate and Nitrite[NO3]- + [NO2]-µmol/lAsmala, Eero
7Nitrite[NO2]-µmol/lAsmala, Eero
8Ammonium[NH4]+µmol/lAsmala, Eero
9Phosphate[PO4]3-µmol/lAsmala, Eero
10SilicateSi(OH)4µmol/lAsmala, Eero
11Nitrate[NO3]-µmol/lAsmala, Eero
12Nitrogen, totalTNµmol/lAsmala, Eero
13Phosphorus, totalTPµmol/lAsmala, Eero
14Nitrogen, total dissolvedTDNµmol/lAsmala, Eero
15Phosphorus, total dissolvedTDPµmol/lAsmala, Eero
16DEPTH, waterDepth watermAsmala, EeroGeocode
17SalinitySalAsmala, EeroPSU
18ConductivityCondmS/cmAsmala, Eero
19Temperature, waterTemp°CAsmala, Eero
20pHpHAsmala, Eero
21Carbon, organic, dissolvedDOCµmol/lAsmala, EeroWet oxidation total organic carbon analyzer Shimadzu
22Carbon, organic, totalTOCµmol/lAsmala, EeroWet oxidation total organic carbon analyzer Shimadzu
23Absorption coefficient, 230 nmac2301/mAsmala, EeroSpectrophotometer UV/VIS (Shimadzu 2401PC)
24Absorption coefficient, 254 nmac2541/mAsmala, EeroSpectrophotometer UV/VIS (Shimadzu 2401PC)
25Absorption coefficient, 275 nmac2751/mAsmala, EeroSpectrophotometer UV/VIS (Shimadzu 2401PC)
26Absorption coefficient, 295 nmac2951/mAsmala, EeroSpectrophotometer UV/VIS (Shimadzu 2401PC)
27Absorption coefficient, 300 nmac3001/mAsmala, EeroSpectrophotometer UV/VIS (Shimadzu 2401PC)
28Absorption coefficient, 350 nmac3501/mAsmala, EeroSpectrophotometer UV/VIS (Shimadzu 2401PC)
29Absorption coefficient, 355 nmac3551/mAsmala, EeroSpectrophotometer UV/VIS (Shimadzu 2401PC)
30Absorption coefficient, 375 nmac3751/mAsmala, EeroSpectrophotometer UV/VIS (Shimadzu 2401PC)
31Absorption coefficient, 400 nmac4001/mAsmala, EeroSpectrophotometer UV/VIS (Shimadzu 2401PC)
32Absorption coefficient, 440 nmac4401/mAsmala, EeroSpectrophotometer UV/VIS (Shimadzu 2401PC)
33Spectral slope, 275-295 nmSpSl 275-295 nm1/µmAsmala, EeroSpectrophotometer UV/VIS (Shimadzu 2401PC)
34Spectral slope, 350-400 nmSpSl 350-400 nm1/µmAsmala, EeroSpectrophotometer UV/VIS (Shimadzu 2401PC)
35RatioRatioAsmala, EeroSpSl 275-295 nm/SpSl 350-400 nm
36Spectral slope, 300-650 nmSpSl 300-650 nm1/µmAsmala, EeroSpectrophotometer UV/VIS (Shimadzu 2401PC)
37Fluorescence, peak TF peak TRUAsmala, EeroVarian Cary Eclipse fluorometer (Agilent)
38Fluorescence, peak AF peak ARUAsmala, EeroVarian Cary Eclipse fluorometer (Agilent)
39Fluorescence, peak MF peak MRUAsmala, EeroVarian Cary Eclipse fluorometer (Agilent)
40Fluorescence, peak CF peak CRUAsmala, EeroVarian Cary Eclipse fluorometer (Agilent)
41Fluorescence indexFIAsmala, EeroVarian Cary Eclipse fluorometer (Agilent)Fluorescence
42Biological indexBIXAsmala, EeroVarian Cary Eclipse fluorometer (Agilent)Fluorescence
43Humification indexHIXAsmala, EeroVarian Cary Eclipse fluorometer (Agilent)Fluorescence
44Chlorophyll aChl aµg/lAsmala, Eero
45δ13C, dissolved organic carbonδ13C DOC‰ PDBAsmala, EeroPDZ Europa ANCA-GSL elemental analyserVPDB
46Molecular massMuAsmala, EeroSEC analyserweight averaged values; 254 nm [Da]
47Nitrogen, inorganic, dissolvedDINµmol/lAsmala, Eero
48Phosphorus, inorganic, dissolvedDIPµmol/lAsmala, Eero
49Nitrogen, organic, dissolvedDONµmol/lAsmala, Eero
50Phosphorus, organic, dissolvedDOPµmol/lAsmala, Eero
51Specific ultraviolet absorbance normalized to DOC, 254 nmSUVA254m2/gAsmala, EeroSpectrophotometer UV/VIS (Shimadzu 2401PC)
Size:
7907 data points

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