Citation:

ame01622

Name: Experiment: Marine fungi may benefit from ocean acidification
Creator: Evamaria Krause
Published: 2013
License: https://creativecommons.org/licenses/by/3.0/
Keywords: Bottles or small containers/Aquaria (<20 L); Coast and continental shelf; Community composition and diversity; Entire community; Laboratory experiment; North Atlantic; Pelagos; Temperate

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Abstract:

Recent studies have discussed the consequences of ocean acidification for bacterial processes and diversity. However, the decomposition of complex substrates in marine environments, a key part of the flow of energy in ecosystems, is largely mediated by marine fungi. Although marine fungi have frequently been reported to prefer low pH levels, this group has been neglected in ocean acidification research. We present the first investigation of direct pH effects on marine fungal abundance and community structure. In microcosm experiments repeated in 2 consecutive years, we incubated natural North Sea water for 4 wk at in situ seawater pH (8.10 and 8.26), pH 7.82 and pH 7.67. Fungal abundance was determined by colony forming unit (cfu) counts, and fungal community structure was investigated by the culture-independent fingerprint method Fungal Automated Ribosomal Intergenic Spacer Analysis (F-ARISA). Furthermore, pH at the study site was determined over a yearly cycle. Fungal cfu were on average 9 times higher at pH 7.82 and 34 times higher at pH 7.67 compared to in situ seawater pH, and we observed fungal community shifts predominantly at pH 7.67. Currently, surface seawater pH at Helgoland Roads remains >8.0 throughout the year; thus we cannot exclude that fungal responses may differ in regions regularly experiencing lower pH values. However, our results suggest that under realistic levels of ocean acidification, marine fungi will reach greater importance in marine biogeochemical cycles. The rise of this group of organisms will affect a variety of biotic interactions in the sea.

Keyword(s):

Bottles or small containers/Aquaria (<20 L); Coast and continental shelf; Community composition and diversity; Entire community; Laboratory experiment; North Atlantic; Pelagos; Temperate

Further details:

Lavigne, Héloïse; Gattuso, Jean-Pierre (2011): seacarb: seawater carbonate chemistry with R. R package version 2.4. https://cran.r-project.org/package=seacarb

Project(s):

Biological Impacts of Ocean Acidification (BIOACID)

Ocean Acidification International Coordination Centre (OA-ICC)

Coverage:

Date/Time Start: 2011-01-01T00:00:00 * Date/Time End: 2012-01-01T00:00:00

Comment:

In order to allow full comparability with other ocean acidification data sets, the R package seacarb (Lavigne and Gattuso, 2011) was used to compute a complete and consistent set of carbonate system variables, as described by Nisumaa et al. (2010). In this dataset the original values were archived in addition with the recalculated parameters (see related PI). The date of carbonate chemistry calculation by seacarb is 2014-04-11.

Parameter(s):

#	Name	Short Name	Unit	Principal Investigator	Method/Device	Comment
1	DATE/TIME	Date/Time				Geocode
2	Incubation duration	Inc dur	weeks	Krause, Evamaria
3	Treatment	Treat		Krause, Evamaria
4	Temperature, water	Temp	°C	Krause, Evamaria
5	Bottle number	Bottle		Krause, Evamaria
6	Replicate	Repl		Krause, Evamaria
7	Colony forming units	CFU	#	Krause, Evamaria
8	Salinity	Sal		Krause, Evamaria
9	Temperature, water	Temp	°C	Krause, Evamaria
10	pH	pH		Krause, Evamaria		NBS scale
11	pH, standard deviation	pH std dev	±	Krause, Evamaria		NBS scale
12	Alkalinity, total	AT	µmol/kg	Krause, Evamaria
13	Alkalinity, total, standard deviation	AT std dev	±	Krause, Evamaria
14	Partial pressure of carbon dioxide (water) at sea surface temperature (wet air)	pCO2water_SST_wet	µatm	Krause, Evamaria
15	Partial pressure of carbon dioxide, standard deviation	pCO2 std dev	±	Krause, Evamaria
16	Carbonate system computation flag	CSC flag		Yang, Yan	Calculated using seacarb after Nisumaa et al. (2010)
17	pH	pH		Yang, Yan	Calculated using seacarb after Nisumaa et al. (2010)	total scale
18	Carbon dioxide	CO2	µmol/kg	Yang, Yan	Calculated using seacarb after Nisumaa et al. (2010)
19	Partial pressure of carbon dioxide (water) at sea surface temperature (wet air)	pCO2water_SST_wet	µatm	Yang, Yan	Calculated using seacarb after Nisumaa et al. (2010)
20	Fugacity of carbon dioxide (water) at sea surface temperature (wet air)	fCO2water_SST_wet	µatm	Yang, Yan	Calculated using seacarb after Nisumaa et al. (2010)
21	Bicarbonate ion	[HCO3]-	µmol/kg	Yang, Yan	Calculated using seacarb after Nisumaa et al. (2010)
22	Carbonate ion	[CO3]2-	µmol/kg	Yang, Yan	Calculated using seacarb after Nisumaa et al. (2010)
23	Carbon, inorganic, dissolved	DIC	µmol/kg	Yang, Yan	Calculated using seacarb after Nisumaa et al. (2010)
24	Aragonite saturation state	Omega Arg		Yang, Yan	Calculated using seacarb after Nisumaa et al. (2010)
25	Calcite saturation state	Omega Cal		Yang, Yan	Calculated using seacarb after Nisumaa et al. (2010)

License:

Creative Commons Attribution 3.0 Unported (CC-BY-3.0)

Status:

Curation Level: Enhanced curation (CurationLevelC)

Size:

8637 data points

Data

Download dataset as tab-delimited text — use the following character encoding:

1 Date/Time	2 Inc dur [weeks]	3 Treat	4 Temp [°C]	5 Bottle	6 Repl	7 CFU [#]	8 Sal	9 Temp [°C]	10 pH (NBS scale)	11 pH std dev [±] (NBS scale)	12 AT [µmol/kg]	13 AT std dev [±]	14 pCO2water_SST_wet [µatm]	15 pCO2 std dev [±]	16 CSC flag	17 pH (total scale)	18 CO2 [µmol/kg]	19 pCO2water_SST_wet [µatm]	20 fCO2water_SST_wet [µatm]	21 [HCO3]- [µmol/kg]	22 [CO3]2- [µmol/kg]	23 DIC [µmol/kg]	24 Omega Arg	25 Omega Cal
2011	2	pH in situ	7	bottle 1	R1	180	30.721	7	8.12	0.00	2366	5	465	5	26	8.01	23	455	453	2105	107	2234	1.63	2.60
2011	2	pH in situ	7	bottle 1	R2	140	30.721	7	8.12	0.00	2366	5	465	5	26	8.01	23	455	453	2105	107	2234	1.63	2.60
2011	2	pH in situ	7	bottle 1	R3	240	30.721	7	8.12	0.00	2366	5	465	5	26	8.01	23	455	453	2105	107	2234	1.63	2.60
2011	2	pH in situ	7	bottle 2	R1	190	30.721	7	8.12	0.00	2366	5	465	5	26	8.01	23	455	453	2105	107	2234	1.63	2.60
2011	2	pH in situ	7	bottle 2	R2	210	30.721	7	8.12	0.00	2366	5	465	5	26	8.01	23	455	453	2105	107	2234	1.63	2.60
2011	2	pH in situ	7	bottle 2	R3	180	30.721	7	8.12	0.00	2366	5	465	5	26	8.01	23	455	453	2105	107	2234	1.63	2.60
2011	2	pH in situ	7	bottle 3	R1	120	30.721	7	8.12	0.00	2366	5	465	5	26	8.01	23	455	453	2105	107	2234	1.63	2.60
2011	2	pH in situ	7	bottle 3	R2	120	30.721	7	8.12	0.00	2366	5	465	5	26	8.01	23	455	453	2105	107	2234	1.63	2.60
2011	2	pH in situ	7	bottle 3	R3	150	30.721	7	8.12	0.00	2366	5	465	5	26	8.01	23	455	453	2105	107	2234	1.63	2.60
2011	2	pH in situ	7	bottle 4	R1	140	30.721	7	8.12	0.00	2366	5	465	5	26	8.01	23	455	453	2105	107	2234	1.63	2.60
2011	2	pH in situ	7	bottle 4	R2	220	30.721	7	8.12	0.00	2366	5	465	5	26	8.01	23	455	453	2105	107	2234	1.63	2.60
2011	2	pH in situ	7	bottle 4	R3	170	30.721	7	8.12	0.00	2366	5	465	5	26	8.01	23	455	453	2105	107	2234	1.63	2.60
2011	2	pH in situ	7	bottle 5	R1	130	30.721	7	8.12	0.00	2366	5	465	5	26	8.01	23	455	453	2105	107	2234	1.63	2.60
2011	2	pH in situ	7	bottle 5	R2	140	30.721	7	8.12	0.00	2366	5	465	5	26	8.01	23	455	453	2105	107	2234	1.63	2.60
2011	2	pH in situ	7	bottle 5	R3	190	30.721	7	8.12	0.00	2366	5	465	5	26	8.01	23	455	453	2105	107	2234	1.63	2.60
2011	2	pH 7.82	7	bottle 1	R1	920	30.721	7	7.81	0.01	2235	11	929	36	26	7.70	46	929	926	2105	52	2204	0.80	1.27
2011	2	pH 7.82	7	bottle 1	R2	920	30.721	7	7.81	0.01	2235	11	929	36	26	7.70	46	929	926	2105	52	2204	0.80	1.27
2011	2	pH 7.82	7	bottle 1	R3	800	30.721	7	7.81	0.01	2235	11	929	36	26	7.70	46	929	926	2105	52	2204	0.80	1.27
2011	2	pH 7.82	7	bottle 2	R1	1390	30.721	7	7.81	0.01	2235	11	929	36	26	7.70	46	929	926	2105	52	2204	0.80	1.27
2011	2	pH 7.82	7	bottle 2	R2	1110	30.721	7	7.81	0.01	2235	11	929	36	26	7.70	46	929	926	2105	52	2204	0.80	1.27
2011	2	pH 7.82	7	bottle 2	R3	1070	30.721	7	7.81	0.01	2235	11	929	36	26	7.70	46	929	926	2105	52	2204	0.80	1.27
2011	2	pH 7.82	7	bottle 3	R1	700	30.721	7	7.81	0.01	2235	11	929	36	26	7.70	46	929	926	2105	52	2204	0.80	1.27
2011	2	pH 7.82	7	bottle 3	R2	680	30.721	7	7.81	0.01	2235	11	929	36	26	7.70	46	929	926	2105	52	2204	0.80	1.27
2011	2	pH 7.82	7	bottle 3	R3	1070	30.721	7	7.81	0.01	2235	11	929	36	26	7.70	46	929	926	2105	52	2204	0.80	1.27
2011	2	pH 7.82	7	bottle 4	R1	940	30.721	7	7.81	0.01	2235	11	929	36	26	7.70	46	929	926	2105	52	2204	0.80	1.27
2011	2	pH 7.82	7	bottle 4	R2	790	30.721	7	7.81	0.01	2235	11	929	36	26	7.70	46	929	926	2105	52	2204	0.80	1.27
2011	2	pH 7.82	7	bottle 4	R3	1080	30.721	7	7.81	0.01	2235	11	929	36	26	7.70	46	929	926	2105	52	2204	0.80	1.27
2011	2	pH 7.82	7	bottle 5	R1	870	30.721	7	7.81	0.01	2235	11	929	36	26	7.70	46	929	926	2105	52	2204	0.80	1.27
2011	2	pH 7.82	7	bottle 5	R2	730	30.721	7	7.81	0.01	2235	11	929	36	26	7.70	46	929	926	2105	52	2204	0.80	1.27
2011	2	pH 7.82	7	bottle 5	R3	710	30.721	7	7.81	0.01	2235	11	929	36	26	7.70	46	929	926	2105	52	2204	0.80	1.27
2011	2	pH 7.67	7	bottle 1	R1	1160	30.721	7	7.70	0.01	2193	2	1208	18	26	7.59	59	1190	1185	2093	40	2192	0.62	0.98
2011	2	pH 7.67	7	bottle 1	R2	990	30.721	7	7.70	0.01	2193	2	1208	18	26	7.59	59	1190	1185	2093	40	2192	0.62	0.98
2011	2	pH 7.67	7	bottle 1	R3	1030	30.721	7	7.70	0.01	2193	2	1208	18	26	7.59	59	1190	1185	2093	40	2192	0.62	0.98
2011	2	pH 7.67	7	bottle 2	R1	1050	30.721	7	7.70	0.01	2193	2	1208	18	26	7.59	59	1190	1185	2093	40	2192	0.62	0.98
2011	2	pH 7.67	7	bottle 2	R2	1200	30.721	7	7.70	0.01	2193	2	1208	18	26	7.59	59	1190	1185	2093	40	2192	0.62	0.98
2011	2	pH 7.67	7	bottle 2	R3	1170	30.721	7	7.70	0.01	2193	2	1208	18	26	7.59	59	1190	1185	2093	40	2192	0.62	0.98
2011	2	pH 7.67	7	bottle 3	R1	1080	30.721	7	7.70	0.01	2193	2	1208	18	26	7.59	59	1190	1185	2093	40	2192	0.62	0.98
2011	2	pH 7.67	7	bottle 3	R2	1560	30.721	7	7.70	0.01	2193	2	1208	18	26	7.59	59	1190	1185	2093	40	2192	0.62	0.98
2011	2	pH 7.67	7	bottle 3	R3	1200	30.721	7	7.70	0.01	2193	2	1208	18	26	7.59	59	1190	1185	2093	40	2192	0.62	0.98
2011	2	pH 7.67	7	bottle 4	R1	1210	30.721	7	7.70	0.01	2193	2	1208	18	26	7.59	59	1190	1185	2093	40	2192	0.62	0.98
2011	2	pH 7.67	7	bottle 4	R2	1180	30.721	7	7.70	0.01	2193	2	1208	18	26	7.59	59	1190	1185	2093	40	2192	0.62	0.98
2011	2	pH 7.67	7	bottle 4	R3	840	30.721	7	7.70	0.01	2193	2	1208	18	26	7.59	59	1190	1185	2093	40	2192	0.62	0.98
2011	2	pH 7.67	7	bottle 5	R1	1040	30.721	7	7.70	0.01	2193	2	1208	18	26	7.59	59	1190	1185	2093	40	2192	0.62	0.98
2011	2	pH 7.67	7	bottle 5	R2	970	30.721	7	7.70	0.01	2193	2	1208	18	26	7.59	59	1190	1185	2093	40	2192	0.62	0.98
2011	2	pH 7.67	7	bottle 5	R3	1110	30.721	7	7.70	0.01	2193	2	1208	18	26	7.59	59	1190	1185	2093	40	2192	0.62	0.98
2011	4	pH in situ	7	bottle 1	R1	180	30.721	7	8.09	0.02	2354	21	498	21	26	7.98	24	489	487	2109	100	2233	1.52	2.43
2011	4	pH in situ	7	bottle 1	R2	100	30.721	7	8.09	0.02	2354	21	498	21	26	7.98	24	489	487	2109	100	2233	1.52	2.43
2011	4	pH in situ	7	bottle 1	R3	100	30.721	7	8.09	0.02	2354	21	498	21	26	7.98	24	489	487	2109	100	2233	1.52	2.43
2011	4	pH in situ	7	bottle 2	R1	80	30.721	7	8.09	0.02	2354	21	498	21	26	7.98	24	489	487	2109	100	2233	1.52	2.43
2011	4	pH in situ	7	bottle 2	R2	90	30.721	7	8.09	0.02	2354	21	498	21	26	7.98	24	489	487	2109	100	2233	1.52	2.43
2011	4	pH in situ	7	bottle 2	R3	90	30.721	7	8.09	0.02	2354	21	498	21	26	7.98	24	489	487	2109	100	2233	1.52	2.43
2011	4	pH in situ	7	bottle 3	R1	60	30.721	7	8.09	0.02	2354	21	498	21	26	7.98	24	489	487	2109	100	2233	1.52	2.43
2011	4	pH in situ	7	bottle 3	R2	130	30.721	7	8.09	0.02	2354	21	498	21	26	7.98	24	489	487	2109	100	2233	1.52	2.43
2011	4	pH in situ	7	bottle 3	R3	80	30.721	7	8.09	0.02	2354	21	498	21	26	7.98	24	489	487	2109	100	2233	1.52	2.43
2011	4	pH in situ	7	bottle 4	R1	130	30.721	7	8.09	0.02	2354	21	498	21	26	7.98	24	489	487	2109	100	2233	1.52	2.43
2011	4	pH in situ	7	bottle 4	R2	160	30.721	7	8.09	0.02	2354	21	498	21	26	7.98	24	489	487	2109	100	2233	1.52	2.43
2011	4	pH in situ	7	bottle 4	R3	160	30.721	7	8.09	0.02	2354	21	498	21	26	7.98	24	489	487	2109	100	2233	1.52	2.43
2011	4	pH in situ	7	bottle 5	R1	50	30.721	7	8.09	0.02	2354	21	498	21	26	7.98	24	489	487	2109	100	2233	1.52	2.43
2011	4	pH in situ	7	bottle 5	R2	80	30.721	7	8.09	0.02	2354	21	498	21	26	7.98	24	489	487	2109	100	2233	1.52	2.43
2011	4	pH in situ	7	bottle 5	R3	90	30.721	7	8.09	0.02	2354	21	498	21	26	7.98	24	489	487	2109	100	2233	1.52	2.43
2011	4	pH 7.82	7	bottle 1	R1	2300	30.721	7	7.79	0.01	2242	12	981	26	26	7.68	49	979	975	2117	50	2216	0.77	1.22
2011	4	pH 7.82	7	bottle 1	R2	3300	30.721	7	7.79	0.01	2242	12	981	26	26	7.68	49	979	975	2117	50	2216	0.77	1.22
2011	4	pH 7.82	7	bottle 1	R3	3400	30.721	7	7.79	0.01	2242	12	981	26	26	7.68	49	979	975	2117	50	2216	0.77	1.22
2011	4	pH 7.82	7	bottle 2	R1	1060	30.721	7	7.79	0.01	2242	12	981	26	26	7.68	49	979	975	2117	50	2216	0.77	1.22
2011	4	pH 7.82	7	bottle 2	R2	880	30.721	7	7.79	0.01	2242	12	981	26	26	7.68	49	979	975	2117	50	2216	0.77	1.22
2011	4	pH 7.82	7	bottle 2	R3	780	30.721	7	7.79	0.01	2242	12	981	26	26	7.68	49	979	975	2117	50	2216	0.77	1.22
2011	4	pH 7.82	7	bottle 3	R1	710	30.721	7	7.79	0.01	2242	12	981	26	26	7.68	49	979	975	2117	50	2216	0.77	1.22
2011	4	pH 7.82	7	bottle 3	R2	940	30.721	7	7.79	0.01	2242	12	981	26	26	7.68	49	979	975	2117	50	2216	0.77	1.22
2011	4	pH 7.82	7	bottle 3	R3	840	30.721	7	7.79	0.01	2242	12	981	26	26	7.68	49	979	975	2117	50	2216	0.77	1.22
2011	4	pH 7.82	7	bottle 4	R1	1020	30.721	7	7.79	0.01	2242	12	981	26	26	7.68	49	979	975	2117	50	2216	0.77	1.22
2011	4	pH 7.82	7	bottle 4	R2	880	30.721	7	7.79	0.01	2242	12	981	26	26	7.68	49	979	975	2117	50	2216	0.77	1.22
2011	4	pH 7.82	7	bottle 4	R3	780	30.721	7	7.79	0.01	2242	12	981	26	26	7.68	49	979	975	2117	50	2216	0.77	1.22
2011	4	pH 7.82	7	bottle 5	R1	1140	30.721	7	7.79	0.01	2242	12	981	26	26	7.68	49	979	975	2117	50	2216	0.77	1.22
2011	4	pH 7.82	7	bottle 5	R2	1160	30.721	7	7.79	0.01	2242	12	981	26	26	7.68	49	979	975	2117	50	2216	0.77	1.22
2011	4	pH 7.82	7	bottle 5	R3	1060	30.721	7	7.79	0.01	2242	12	981	26	26	7.68	49	979	975	2117	50	2216	0.77	1.22
2011	4	pH 7.67	7	bottle 1	R1	1650	30.721	7	7.69	0.01	2203	9	1246	43	26	7.58	61	1225	1220	2104	40	2205	0.61	0.97
2011	4	pH 7.67	7	bottle 1	R2	1590	30.721	7	7.69	0.01	2203	9	1246	43	26	7.58	61	1225	1220	2104	40	2205	0.61	0.97
2011	4	pH 7.67	7	bottle 1	R3	1710	30.721	7	7.69	0.01	2203	9	1246	43	26	7.58	61	1225	1220	2104	40	2205	0.61	0.97
2011	4	pH 7.67	7	bottle 2	R1	10400	30.721	7	7.69	0.01	2203	9	1246	43	26	7.58	61	1225	1220	2104	40	2205	0.61	0.97
2011	4	pH 7.67	7	bottle 2	R2	8800	30.721	7	7.69	0.01	2203	9	1246	43	26	7.58	61	1225	1220	2104	40	2205	0.61	0.97
2011	4	pH 7.67	7	bottle 2	R3	7800	30.721	7	7.69	0.01	2203	9	1246	43	26	7.58	61	1225	1220	2104	40	2205	0.61	0.97
2011	4	pH 7.67	7	bottle 3	R1	9600	30.721	7	7.69	0.01	2203	9	1246	43	26	7.58	61	1225	1220	2104	40	2205	0.61	0.97
2011	4	pH 7.67	7	bottle 3	R2	10800	30.721	7	7.69	0.01	2203	9	1246	43	26	7.58	61	1225	1220	2104	40	2205	0.61	0.97
2011	4	pH 7.67	7	bottle 3	R3	7200	30.721	7	7.69	0.01	2203	9	1246	43	26	7.58	61	1225	1220	2104	40	2205	0.61	0.97
2011	4	pH 7.67	7	bottle 4	R1	8600	30.721	7	7.69	0.01	2203	9	1246	43	26	7.58	61	1225	1220	2104	40	2205	0.61	0.97
2011	4	pH 7.67	7	bottle 4	R2	6600	30.721	7	7.69	0.01	2203	9	1246	43	26	7.58	61	1225	1220	2104	40	2205	0.61	0.97
2011	4	pH 7.67	7	bottle 4	R3	9000	30.721	7	7.69	0.01	2203	9	1246	43	26	7.58	61	1225	1220	2104	40	2205	0.61	0.97
2011	4	pH 7.67	7	bottle 5	R1	8400	30.721	7	7.69	0.01	2203	9	1246	43	26	7.58	61	1225	1220	2104	40	2205	0.61	0.97
2011	4	pH 7.67	7	bottle 5	R2	10200	30.721	7	7.69	0.01	2203	9	1246	43	26	7.58	61	1225	1220	2104	40	2205	0.61	0.97
2011	4	pH 7.67	7	bottle 5	R3	9200	30.721	7	7.69	0.01	2203	9	1246	43	26	7.58	61	1225	1220	2104	40	2205	0.61	0.97
2011	2	pH in situ	18	bottle 1	R1	920	30.721	7	8.12	0.00	2366	5	465	5	26	8.01	23	455	453	2105	107	2234	1.63	2.60
2011	2	pH in situ	18	bottle 1	R2	890	30.721	7	8.12	0.00	2366	5	465	5	26	8.01	23	455	453	2105	107	2234	1.63	2.60
2011	2	pH in situ	18	bottle 1	R3	1000	30.721	7	8.12	0.00	2366	5	465	5	26	8.01	23	455	453	2105	107	2234	1.63	2.60
2011	2	pH in situ	18	bottle 2	R1	850	30.721	7	8.12	0.00	2366	5	465	5	26	8.01	23	455	453	2105	107	2234	1.63	2.60
2011	2	pH in situ	18	bottle 2	R2	850	30.721	7	8.12	0.00	2366	5	465	5	26	8.01	23	455	453	2105	107	2234	1.63	2.60
2011	2	pH in situ	18	bottle 2	R3	1080	30.721	7	8.12	0.00	2366	5	465	5	26	8.01	23	455	453	2105	107	2234	1.63	2.60
2011	2	pH in situ	18	bottle 3	R1	820	30.721	7	8.12	0.00	2366	5	465	5	26	8.01	23	455	453	2105	107	2234	1.63	2.60
2011	2	pH in situ	18	bottle 3	R2	910	30.721	7	8.12	0.00	2366	5	465	5	26	8.01	23	455	453	2105	107	2234	1.63	2.60
2011	2	pH in situ	18	bottle 3	R3	1040	30.721	7	8.12	0.00	2366	5	465	5	26	8.01	23	455	453	2105	107	2234	1.63	2.60
2011	2	pH in situ	18	bottle 4	R1	860	30.721	7	8.12	0.00	2366	5	465	5	26	8.01	23	455	453	2105	107	2234	1.63	2.60
2011	2	pH in situ	18	bottle 4	R2	820	30.721	7	8.12	0.00	2366	5	465	5	26	8.01	23	455	453	2105	107	2234	1.63	2.60
2011	2	pH in situ	18	bottle 4	R3	880	30.721	7	8.12	0.00	2366	5	465	5	26	8.01	23	455	453	2105	107	2234	1.63	2.60
2011	2	pH in situ	18	bottle 5	R1	1180	30.721	7	8.12	0.00	2366	5	465	5	26	8.01	23	455	453	2105	107	2234	1.63	2.60
2011	2	pH in situ	18	bottle 5	R2	1090	30.721	7	8.12	0.00	2366	5	465	5	26	8.01	23	455	453	2105	107	2234	1.63	2.60
2011	2	pH in situ	18	bottle 5	R3	1160	30.721	7	8.12	0.00	2366	5	465	5	26	8.01	23	455	453	2105	107	2234	1.63	2.60
2011	2	pH 7.82	18	bottle 1	R1	12500	30.721	7	7.81	0.01	2235	11	929	36	26	7.70	46	929	926	2105	52	2204	0.80	1.27
2011	2	pH 7.82	18	bottle 1	R2	11300	30.721	7	7.81	0.01	2235	11	929	36	26	7.70	46	929	926	2105	52	2204	0.80	1.27
2011	2	pH 7.82	18	bottle 1	R3	11700	30.721	7	7.81	0.01	2235	11	929	36	26	7.70	46	929	926	2105	52	2204	0.80	1.27
2011	2	pH 7.82	18	bottle 2	R1	14200	30.721	7	7.81	0.01	2235	11	929	36	26	7.70	46	929	926	2105	52	2204	0.80	1.27
2011	2	pH 7.82	18	bottle 2	R2	14800	30.721	7	7.81	0.01	2235	11	929	36	26	7.70	46	929	926	2105	52	2204	0.80	1.27
2011	2	pH 7.82	18	bottle 2	R3	15500	30.721	7	7.81	0.01	2235	11	929	36	26	7.70	46	929	926	2105	52	2204	0.80	1.27
2011	2	pH 7.82	18	bottle 3	R1	14200	30.721	7	7.81	0.01	2235	11	929	36	26	7.70	46	929	926	2105	52	2204	0.80	1.27
2011	2	pH 7.82	18	bottle 3	R2	12700	30.721	7	7.81	0.01	2235	11	929	36	26	7.70	46	929	926	2105	52	2204	0.80	1.27
2011	2	pH 7.82	18	bottle 3	R3	14200	30.721	7	7.81	0.01	2235	11	929	36	26	7.70	46	929	926	2105	52	2204	0.80	1.27
2011	2	pH 7.82	18	bottle 4	R1	14600	30.721	7	7.81	0.01	2235	11	929	36	26	7.70	46	929	926	2105	52	2204	0.80	1.27
2011	2	pH 7.82	18	bottle 4	R2	9800	30.721	7	7.81	0.01	2235	11	929	36	26	7.70	46	929	926	2105	52	2204	0.80	1.27
2011	2	pH 7.82	18	bottle 4	R3	12300	30.721	7	7.81	0.01	2235	11	929	36	26	7.70	46	929	926	2105	52	2204	0.80	1.27
2011	2	pH 7.82	18	bottle 5	R1	10700	30.721	7	7.81	0.01	2235	11	929	36	26	7.70	46	929	926	2105	52	2204	0.80	1.27
2011	2	pH 7.82	18	bottle 5	R2	10100	30.721	7	7.81	0.01	2235	11	929	36	26	7.70	46	929	926	2105	52	2204	0.80	1.27
2011	2	pH 7.82	18	bottle 5	R3	10400	30.721	7	7.81	0.01	2235	11	929	36	26	7.70	46	929	926	2105	52	2204	0.80	1.27
2011	2	pH 7.67	18	bottle 1	R1	46000	30.721	7	7.70	0.01	2193	2	1208	18	26	7.59	59	1190	1185	2093	40	2192	0.62	0.98
2011	2	pH 7.67	18	bottle 1	R2	48000	30.721	7	7.70	0.01	2193	2	1208	18	26	7.59	59	1190	1185	2093	40	2192	0.62	0.98
2011	2	pH 7.67	18	bottle 1	R3	26000	30.721	7	7.70	0.01	2193	2	1208	18	26	7.59	59	1190	1185	2093	40	2192	0.62	0.98
2011	2	pH 7.67	18	bottle 2	R1	64000	30.721	7	7.70	0.01	2193	2	1208	18	26	7.59	59	1190	1185	2093	40	2192	0.62	0.98
2011	2	pH 7.67	18	bottle 2	R2	32000	30.721	7	7.70	0.01	2193	2	1208	18	26	7.59	59	1190	1185	2093	40	2192	0.62	0.98
2011	2	pH 7.67	18	bottle 2	R3	24000	30.721	7	7.70	0.01	2193	2	1208	18	26	7.59	59	1190	1185	2093	40	2192	0.62	0.98
2011	2	pH 7.67	18	bottle 3	R1	42000	30.721	7	7.70	0.01	2193	2	1208	18	26	7.59	59	1190	1185	2093	40	2192	0.62	0.98
2011	2	pH 7.67	18	bottle 3	R2	36000	30.721	7	7.70	0.01	2193	2	1208	18	26	7.59	59	1190	1185	2093	40	2192	0.62	0.98
2011	2	pH 7.67	18	bottle 3	R3	38000	30.721	7	7.70	0.01	2193	2	1208	18	26	7.59	59	1190	1185	2093	40	2192	0.62	0.98
2011	2	pH 7.67	18	bottle 4	R1	60000	30.721	7	7.70	0.01	2193	2	1208	18	26	7.59	59	1190	1185	2093	40	2192	0.62	0.98
2011	2	pH 7.67	18	bottle 4	R2	40000	30.721	7	7.70	0.01	2193	2	1208	18	26	7.59	59	1190	1185	2093	40	2192	0.62	0.98
2011	2	pH 7.67	18	bottle 4	R3	38000	30.721	7	7.70	0.01	2193	2	1208	18	26	7.59	59	1190	1185	2093	40	2192	0.62	0.98
2011	2	pH 7.67	18	bottle 5	R1	44000	30.721	7	7.70	0.01	2193	2	1208	18	26	7.59	59	1190	1185	2093	40	2192	0.62	0.98
2011	2	pH 7.67	18	bottle 5	R2	52000	30.721	7	7.70	0.01	2193	2	1208	18	26	7.59	59	1190	1185	2093	40	2192	0.62	0.98
2011	2	pH 7.67	18	bottle 5	R3	56000	30.721	7	7.70	0.01	2193	2	1208	18	26	7.59	59	1190	1185	2093	40	2192	0.62	0.98
2011	4	pH in situ	18	bottle 1	R1	780	30.721	7	8.09	0.02	2354	21	498	21	26	7.98	24	489	487	2109	100	2233	1.52	2.43
2011	4	pH in situ	18	bottle 1	R2	1030	30.721	7	8.09	0.02	2354	21	498	21	26	7.98	24	489	487	2109	100	2233	1.52	2.43
2011	4	pH in situ	18	bottle 1	R3	800	30.721	7	8.09	0.02	2354	21	498	21	26	7.98	24	489	487	2109	100	2233	1.52	2.43
2011	4	pH in situ	18	bottle 2	R1	1060	30.721	7	8.09	0.02	2354	21	498	21	26	7.98	24	489	487	2109	100	2233	1.52	2.43
2011	4	pH in situ	18	bottle 2	R2	820	30.721	7	8.09	0.02	2354	21	498	21	26	7.98	24	489	487	2109	100	2233	1.52	2.43
2011	4	pH in situ	18	bottle 2	R3	940	30.721	7	8.09	0.02	2354	21	498	21	26	7.98	24	489	487	2109	100	2233	1.52	2.43
2011	4	pH in situ	18	bottle 3	R1	840	30.721	7	8.09	0.02	2354	21	498	21	26	7.98	24	489	487	2109	100	2233	1.52	2.43
2011	4	pH in situ	18	bottle 3	R2	560	30.721	7	8.09	0.02	2354	21	498	21	26	7.98	24	489	487	2109	100	2233	1.52	2.43
2011	4	pH in situ	18	bottle 3	R3	620	30.721	7	8.09	0.02	2354	21	498	21	26	7.98	24	489	487	2109	100	2233	1.52	2.43
2011	4	pH in situ	18	bottle 4	R1	870	30.721	7	8.09	0.02	2354	21	498	21	26	7.98	24	489	487	2109	100	2233	1.52	2.43
2011	4	pH in situ	18	bottle 4	R2	1010	30.721	7	8.09	0.02	2354	21	498	21	26	7.98	24	489	487	2109	100	2233	1.52	2.43
2011	4	pH in situ	18	bottle 4	R3	910	30.721	7	8.09	0.02	2354	21	498	21	26	7.98	24	489	487	2109	100	2233	1.52	2.43
2011	4	pH in situ	18	bottle 5	R1	540	30.721	7	8.09	0.02	2354	21	498	21	26	7.98	24	489	487	2109	100	2233	1.52	2.43
2011	4	pH in situ	18	bottle 5	R2	660	30.721	7	8.09	0.02	2354	21	498	21	26	7.98	24	489	487	2109	100	2233	1.52	2.43
2011	4	pH in situ	18	bottle 5	R3	610	30.721	7	8.09	0.02	2354	21	498	21	26	7.98	24	489	487	2109	100	2233	1.52	2.43
2011	4	pH 7.82	18	bottle 1	R1	8200	30.721	7	7.79	0.01	2242	12	981	26	26	7.68	49	979	975	2117	50	2216	0.77	1.22
2011	4	pH 7.82	18	bottle 1	R2	6600	30.721	7	7.79	0.01	2242	12	981	26	26	7.68	49	979	975	2117	50	2216	0.77	1.22
2011	4	pH 7.82	18	bottle 1	R3	7600	30.721	7	7.79	0.01	2242	12	981	26	26	7.68	49	979	975	2117	50	2216	0.77	1.22
2011	4	pH 7.82	18	bottle 2	R1	7800	30.721	7	7.79	0.01	2242	12	981	26	26	7.68	49	979	975	2117	50	2216	0.77	1.22
2011	4	pH 7.82	18	bottle 2	R2	6100	30.721	7	7.79	0.01	2242	12	981	26	26	7.68	49	979	975	2117	50	2216	0.77	1.22
2011	4	pH 7.82	18	bottle 2	R3	6200	30.721	7	7.79	0.01	2242	12	981	26	26	7.68	49	979	975	2117	50	2216	0.77	1.22
2011	4	pH 7.82	18	bottle 3	R1	9200	30.721	7	7.79	0.01	2242	12	981	26	26	7.68	49	979	975	2117	50	2216	0.77	1.22
2011	4	pH 7.82	18	bottle 3	R2	5700	30.721	7	7.79	0.01	2242	12	981	26	26	7.68	49	979	975	2117	50	2216	0.77	1.22
2011	4	pH 7.82	18	bottle 3	R3	4300	30.721	7	7.79	0.01	2242	12	981	26	26	7.68	49	979	975	2117	50	2216	0.77	1.22
2011	4	pH 7.82	18	bottle 4	R1	8300	30.721	7	7.79	0.01	2242	12	981	26	26	7.68	49	979	975	2117	50	2216	0.77	1.22
2011	4	pH 7.82	18	bottle 4	R2	6600	30.721	7	7.79	0.01	2242	12	981	26	26	7.68	49	979	975	2117	50	2216	0.77	1.22
2011	4	pH 7.82	18	bottle 4	R3	6300	30.721	7	7.79	0.01	2242	12	981	26	26	7.68	49	979	975	2117	50	2216	0.77	1.22
2011	4	pH 7.82	18	bottle 5	R1	6700	30.721	7	7.79	0.01	2242	12	981	26	26	7.68	49	979	975	2117	50	2216	0.77	1.22
2011	4	pH 7.82	18	bottle 5	R2	5300	30.721	7	7.79	0.01	2242	12	981	26	26	7.68	49	979	975	2117	50	2216	0.77	1.22
2011	4	pH 7.82	18	bottle 5	R3	7100	30.721	7	7.79	0.01	2242	12	981	26	26	7.68	49	979	975	2117	50	2216	0.77	1.22
2011	4	pH 7.67	18	bottle 1	R1		30.721	7	7.69	0.01	2203	9	1246	43	26	7.58	61	1225	1220	2104	40	2205	0.61	0.97
2011	4	pH 7.67	18	bottle 1	R2		30.721	7	7.69	0.01	2203	9	1246	43	26	7.58	61	1225	1220	2104	40	2205	0.61	0.97
2011	4	pH 7.67	18	bottle 1	R3		30.721	7	7.69	0.01	2203	9	1246	43	26	7.58	61	1225	1220	2104	40	2205	0.61	0.97
2011	4	pH 7.67	18	bottle 2	R1	90000	30.721	7	7.69	0.01	2203	9	1246	43	26	7.58	61	1225	1220	2104	40	2205	0.61	0.97
2011	4	pH 7.67	18	bottle 2	R2	40000	30.721	7	7.69	0.01	2203	9	1246	43	26	7.58	61	1225	1220	2104	40	2205	0.61	0.97
2011	4	pH 7.67	18	bottle 2	R3	24000	30.721	7	7.69	0.01	2203	9	1246	43	26	7.58	61	1225	1220	2104	40	2205	0.61	0.97
2011	4	pH 7.67	18	bottle 3	R1	24000	30.721	7	7.69	0.01	2203	9	1246	43	26	7.58	61	1225	1220	2104	40	2205	0.61	0.97
2011	4	pH 7.67	18	bottle 3	R2	10000	30.721	7	7.69	0.01	2203	9	1246	43	26	7.58	61	1225	1220	2104	40	2205	0.61	0.97
2011	4	pH 7.67	18	bottle 3	R3	18000	30.721	7	7.69	0.01	2203	9	1246	43	26	7.58	61	1225	1220	2104	40	2205	0.61	0.97
2011	4	pH 7.67	18	bottle 4	R1	38000	30.721	7	7.69	0.01	2203	9	1246	43	26	7.58	61	1225	1220	2104	40	2205	0.61	0.97
2011	4	pH 7.67	18	bottle 4	R2	16000	30.721	7	7.69	0.01	2203	9	1246	43	26	7.58	61	1225	1220	2104	40	2205	0.61	0.97
2011	4	pH 7.67	18	bottle 4	R3	18000	30.721	7	7.69	0.01	2203	9	1246	43	26	7.58	61	1225	1220	2104	40	2205	0.61	0.97
2011	4	pH 7.67	18	bottle 5	R1	16000	30.721	7	7.69	0.01	2203	9	1246	43	26	7.58	61	1225	1220	2104	40	2205	0.61	0.97
2011	4	pH 7.67	18	bottle 5	R2	6000	30.721	7	7.69	0.01	2203	9	1246	43	26	7.58	61	1225	1220	2104	40	2205	0.61	0.97
2011	4	pH 7.67	18	bottle 5	R3	8000	30.721	7	7.69	0.01	2203	9	1246	43	26	7.58	61	1225	1220	2104	40	2205	0.61	0.97
2012	2	pH in situ	8	bottle 1	R1	570	33.441	8	8.18	0.01	2328	6	397	10	26	8.08	18	374	372	2004	131	2152	1.98	3.14
2012	2	pH in situ	8	bottle 1	R2	120	33.441	8	8.18	0.01	2328	6	397	10	26	8.08	18	374	372	2004	131	2152	1.98	3.14
2012	2	pH in situ	8	bottle 1	R3	210	33.441	8	8.18	0.01	2328	6	397	10	26	8.08	18	374	372	2004	131	2152	1.98	3.14
2012	2	pH in situ	8	bottle 2	R1	420	33.441	8	8.18	0.01	2328	6	397	10	26	8.08	18	374	372	2004	131	2152	1.98	3.14
2012	2	pH in situ	8	bottle 2	R2	400	33.441	8	8.18	0.01	2328	6	397	10	26	8.08	18	374	372	2004	131	2152	1.98	3.14
2012	2	pH in situ	8	bottle 2	R3	30	33.441	8	8.18	0.01	2328	6	397	10	26	8.08	18	374	372	2004	131	2152	1.98	3.14
2012	2	pH in situ	8	bottle 3	R1	410	33.441	8	8.18	0.01	2328	6	397	10	26	8.08	18	374	372	2004	131	2152	1.98	3.14
2012	2	pH in situ	8	bottle 3	R2	460	33.441	8	8.18	0.01	2328	6	397	10	26	8.08	18	374	372	2004	131	2152	1.98	3.14
2012	2	pH in situ	8	bottle 3	R3	500	33.441	8	8.18	0.01	2328	6	397	10	26	8.08	18	374	372	2004	131	2152	1.98	3.14
2012	2	pH in situ	8	bottle 4	R1	230	33.441	8	8.18	0.01	2328	6	397	10	26	8.08	18	374	372	2004	131	2152	1.98	3.14
2012	2	pH in situ	8	bottle 4	R2	250	33.441	8	8.18	0.01	2328	6	397	10	26	8.08	18	374	372	2004	131	2152	1.98	3.14
2012	2	pH in situ	8	bottle 4	R3	350	33.441	8	8.18	0.01	2328	6	397	10	26	8.08	18	374	372	2004	131	2152	1.98	3.14
2012	2	pH in situ	8	bottle 5	R1	390	33.441	8	8.18	0.01	2328	6	397	10	26	8.08	18	374	372	2004	131	2152	1.98	3.14
2012	2	pH in situ	8	bottle 5	R2	430	33.441	8	8.18	0.01	2328	6	397	10	26	8.08	18	374	372	2004	131	2152	1.98	3.14
2012	2	pH in situ	8	bottle 5	R3	260	33.441	8	8.18	0.01	2328	6	397	10	26	8.08	18	374	372	2004	131	2152	1.98	3.14
2012	2	pH 7.82	8	bottle 1	R1	3100	33.441	8	7.76	0.01	2163	12	1052	24	26	7.66	47	998	994	2036	50	2133	0.77	1.21
2012	2	pH 7.82	8	bottle 1	R2	2700	33.441	8	7.76	0.01	2163	12	1052	24	26	7.66	47	998	994	2036	50	2133	0.77	1.21
2012	2	pH 7.82	8	bottle 1	R3	3300	33.441	8	7.76	0.01	2163	12	1052	24	26	7.66	47	998	994	2036	50	2133	0.77	1.21
2012	2	pH 7.82	8	bottle 2	R1	3000	33.441	8	7.76	0.01	2163	12	1052	24	26	7.66	47	998	994	2036	50	2133	0.77	1.21
2012	2	pH 7.82	8	bottle 2	R2	4300	33.441	8	7.76	0.01	2163	12	1052	24	26	7.66	47	998	994	2036	50	2133	0.77	1.21
2012	2	pH 7.82	8	bottle 2	R3	3400	33.441	8	7.76	0.01	2163	12	1052	24	26	7.66	47	998	994	2036	50	2133	0.77	1.21
2012	2	pH 7.82	8	bottle 3	R1	3500	33.441	8	7.76	0.01	2163	12	1052	24	26	7.66	47	998	994	2036	50	2133	0.77	1.21
2012	2	pH 7.82	8	bottle 3	R2	3000	33.441	8	7.76	0.01	2163	12	1052	24	26	7.66	47	998	994	2036	50	2133	0.77	1.21
2012	2	pH 7.82	8	bottle 3	R3	3500	33.441	8	7.76	0.01	2163	12	1052	24	26	7.66	47	998	994	2036	50	2133	0.77	1.21
2012	2	pH 7.82	8	bottle 4	R1	2800	33.441	8	7.76	0.01	2163	12	1052	24	26	7.66	47	998	994	2036	50	2133	0.77	1.21
2012	2	pH 7.82	8	bottle 4	R2	3000	33.441	8	7.76	0.01	2163	12	1052	24	26	7.66	47	998	994	2036	50	2133	0.77	1.21
2012	2	pH 7.82	8	bottle 4	R3	4000	33.441	8	7.76	0.01	2163	12	1052	24	26	7.66	47	998	994	2036	50	2133	0.77	1.21
2012	2	pH 7.82	8	bottle 5	R1	6300	33.441	8	7.76	0.01	2163	12	1052	24	26	7.66	47	998	994	2036	50	2133	0.77	1.21
2012	2	pH 7.82	8	bottle 5	R2	4300	33.441	8	7.76	0.01	2163	12	1052	24	26	7.66	47	998	994	2036	50	2133	0.77	1.21
2012	2	pH 7.82	8	bottle 5	R3	4500	33.441	8	7.76	0.01	2163	12	1052	24	26	7.66	47	998	994	2036	50	2133	0.77	1.21
2012	2	pH 7.67	8	bottle 1	R1	11800	33.441	8	7.62	0.01	2099	12	1442	37	26	7.52	64	1359	1353	2007	36	2108	0.55	0.87
2012	2	pH 7.67	8	bottle 1	R2	10900	33.441	8	7.62	0.01	2099	12	1442	37	26	7.52	64	1359	1353	2007	36	2108	0.55	0.87
2012	2	pH 7.67	8	bottle 1	R3	12200	33.441	8	7.62	0.01	2099	12	1442	37	26	7.52	64	1359	1353	2007	36	2108	0.55	0.87
2012	2	pH 7.67	8	bottle 2	R1	14100	33.441	8	7.62	0.01	2099	12	1442	37	26	7.52	64	1359	1353	2007	36	2108	0.55	0.87
2012	2	pH 7.67	8	bottle 2	R2	4700	33.441	8	7.62	0.01	2099	12	1442	37	26	7.52	64	1359	1353	2007	36	2108	0.55	0.87
2012	2	pH 7.67	8	bottle 2	R3	12300	33.441	8	7.62	0.01	2099	12	1442	37	26	7.52	64	1359	1353	2007	36	2108	0.55	0.87
2012	2	pH 7.67	8	bottle 3	R1	13700	33.441	8	7.62	0.01	2099	12	1442	37	26	7.52	64	1359	1353	2007	36	2108	0.55	0.87
2012	2	pH 7.67	8	bottle 3	R2	13000	33.441	8	7.62	0.01	2099	12	1442	37	26	7.52	64	1359	1353	2007	36	2108	0.55	0.87
2012	2	pH 7.67	8	bottle 3	R3	11500	33.441	8	7.62	0.01	2099	12	1442	37	26	7.52	64	1359	1353	2007	36	2108	0.55	0.87
2012	2	pH 7.67	8	bottle 4	R1	7500	33.441	8	7.62	0.01	2099	12	1442	37	26	7.52	64	1359	1353	2007	36	2108	0.55	0.87
2012	2	pH 7.67	8	bottle 4	R2	6200	33.441	8	7.62	0.01	2099	12	1442	37	26	7.52	64	1359	1353	2007	36	2108	0.55	0.87
2012	2	pH 7.67	8	bottle 4	R3	6400	33.441	8	7.62	0.01	2099	12	1442	37	26	7.52	64	1359	1353	2007	36	2108	0.55	0.87
2012	2	pH 7.67	8	bottle 5	R1	6100	33.441	8	7.62	0.01	2099	12	1442	37	26	7.52	64	1359	1353	2007	36	2108	0.55	0.87
2012	2	pH 7.67	8	bottle 5	R2	10000	33.441	8	7.62	0.01	2099	12	1442	37	26	7.52	64	1359	1353	2007	36	2108	0.55	0.87
2012	2	pH 7.67	8	bottle 5	R3	9700	33.441	8	7.62	0.01	2099	12	1442	37	26	7.52	64	1359	1353	2007	36	2108	0.55	0.87
2012	4	pH in situ	8	bottle 1	R1	230	33.441	8	8.14	0.01	2327	9	406	14	26	8.04	20	415	413	2028	120	2168	1.83	2.90
2012	4	pH in situ	8	bottle 1	R2	210	33.441	8	8.14	0.01	2327	9	406	14	26	8.04	20	415	413	2028	120	2168	1.83	2.90
2012	4	pH in situ	8	bottle 1	R3	130	33.441	8	8.14	0.01	2327	9	406	14	26	8.04	20	415	413	2028	120	2168	1.83	2.90
2012	4	pH in situ	8	bottle 2	R1	240	33.441	8	8.14	0.01	2327	9	406	14	26	8.04	20	415	413	2028	120	2168	1.83	2.90
2012	4	pH in situ	8	bottle 2	R2	30	33.441	8	8.14	0.01	2327	9	406	14	26	8.04	20	415	413	2028	120	2168	1.83	2.90
2012	4	pH in situ	8	bottle 2	R3	260	33.441	8	8.14	0.01	2327	9	406	14	26	8.04	20	415	413	2028	120	2168	1.83	2.90
2012	4	pH in situ	8	bottle 3	R1	160	33.441	8	8.14	0.01	2327	9	406	14	26	8.04	20	415	413	2028	120	2168	1.83	2.90
2012	4	pH in situ	8	bottle 3	R2	130	33.441	8	8.14	0.01	2327	9	406	14	26	8.04	20	415	413	2028	120	2168	1.83	2.90
2012	4	pH in situ	8	bottle 3	R3	70	33.441	8	8.14	0.01	2327	9	406	14	26	8.04	20	415	413	2028	120	2168	1.83	2.90
2012	4	pH in situ	8	bottle 4	R1	230	33.441	8	8.14	0.01	2327	9	406	14	26	8.04	20	415	413	2028	120	2168	1.83	2.90
2012	4	pH in situ	8	bottle 4	R2	140	33.441	8	8.14	0.01	2327	9	406	14	26	8.04	20	415	413	2028	120	2168	1.83	2.90
2012	4	pH in situ	8	bottle 4	R3	130	33.441	8	8.14	0.01	2327	9	406	14	26	8.04	20	415	413	2028	120	2168	1.83	2.90
2012	4	pH in situ	8	bottle 5	R1	130	33.441	8	8.14	0.01	2327	9	406	14	26	8.04	20	415	413	2028	120	2168	1.83	2.90
2012	4	pH in situ	8	bottle 5	R2	80	33.441	8	8.14	0.01	2327	9	406	14	26	8.04	20	415	413	2028	120	2168	1.83	2.90
2012	4	pH in situ	8	bottle 5	R3	60	33.441	8	8.14	0.01	2327	9	406	14	26	8.04	20	415	413	2028	120	2168	1.83	2.90
2012	4	pH 7.82	8	bottle 1	R1	1860	33.441	8	7.70	0.01	2158	8	1139	40	26	7.60	54	1152	1148	2046	44	2145	0.67	1.06
2012	4	pH 7.82	8	bottle 1	R2	2540	33.441	8	7.70	0.01	2158	8	1139	40	26	7.60	54	1152	1148	2046	44	2145	0.67	1.06
2012	4	pH 7.82	8	bottle 1	R3	2030	33.441	8	7.70	0.01	2158	8	1139	40	26	7.60	54	1152	1148	2046	44	2145	0.67	1.06
2012	4	pH 7.82	8	bottle 2	R1	780	33.441	8	7.70	0.01	2158	8	1139	40	26	7.60	54	1152	1148	2046	44	2145	0.67	1.06
2012	4	pH 7.82	8	bottle 2	R2	560	33.441	8	7.70	0.01	2158	8	1139	40	26	7.60	54	1152	1148	2046	44	2145	0.67	1.06
2012	4	pH 7.82	8	bottle 2	R3	760	33.441	8	7.70	0.01	2158	8	1139	40	26	7.60	54	1152	1148	2046	44	2145	0.67	1.06
2012	4	pH 7.82	8	bottle 3	R1	1150	33.441	8	7.70	0.01	2158	8	1139	40	26	7.60	54	1152	1148	2046	44	2145	0.67	1.06
2012	4	pH 7.82	8	bottle 3	R2	1500	33.441	8	7.70	0.01	2158	8	1139	40	26	7.60	54	1152	1148	2046	44	2145	0.67	1.06
2012	4	pH 7.82	8	bottle 3	R3	1250	33.441	8	7.70	0.01	2158	8	1139	40	26	7.60	54	1152	1148	2046	44	2145	0.67	1.06
2012	4	pH 7.82	8	bottle 4	R1	1520	33.441	8	7.70	0.01	2158	8	1139	40	26	7.60	54	1152	1148	2046	44	2145	0.67	1.06
2012	4	pH 7.82	8	bottle 4	R2	1610	33.441	8	7.70	0.01	2158	8	1139	40	26	7.60	54	1152	1148	2046	44	2145	0.67	1.06
2012	4	pH 7.82	8	bottle 4	R3	1830	33.441	8	7.70	0.01	2158	8	1139	40	26	7.60	54	1152	1148	2046	44	2145	0.67	1.06
2012	4	pH 7.82	8	bottle 5	R1	860	33.441	8	7.70	0.01	2158	8	1139	40	26	7.60	54	1152	1148	2046	44	2145	0.67	1.06
2012	4	pH 7.82	8	bottle 5	R2	910	33.441	8	7.70	0.01	2158	8	1139	40	26	7.60	54	1152	1148	2046	44	2145	0.67	1.06
2012	4	pH 7.82	8	bottle 5	R3	870	33.441	8	7.70	0.01	2158	8	1139	40	26	7.60	54	1152	1148	2046	44	2145	0.67	1.06
2012	4	pH 7.67	8	bottle 1	R1	4900	33.441	8	7.58	0.01	2113	6	1482	46	26	7.48	71	1506	1500	2029	33	2133	0.50	0.80
2012	4	pH 7.67	8	bottle 1	R2	5200	33.441	8	7.58	0.01	2113	6	1482	46	26	7.48	71	1506	1500	2029	33	2133	0.50	0.80
2012	4	pH 7.67	8	bottle 1	R3	4700	33.441	8	7.58	0.01	2113	6	1482	46	26	7.48	71	1506	1500	2029	33	2133	0.50	0.80
2012	4	pH 7.67	8	bottle 2	R1	8400	33.441	8	7.58	0.01	2113	6	1482	46	26	7.48	71	1506	1500	2029	33	2133	0.50	0.80
2012	4	pH 7.67	8	bottle 2	R2	5200	33.441	8	7.58	0.01	2113	6	1482	46	26	7.48	71	1506	1500	2029	33	2133	0.50	0.80
2012	4	pH 7.67	8	bottle 2	R3	5700	33.441	8	7.58	0.01	2113	6	1482	46	26	7.48	71	1506	1500	2029	33	2133	0.50	0.80
2012	4	pH 7.67	8	bottle 3	R1	3600	33.441	8	7.58	0.01	2113	6	1482	46	26	7.48	71	1506	1500	2029	33	2133	0.50	0.80
2012	4	pH 7.67	8	bottle 3	R2	5800	33.441	8	7.58	0.01	2113	6	1482	46	26	7.48	71	1506	1500	2029	33	2133	0.50	0.80
2012	4	pH 7.67	8	bottle 3	R3	5600	33.441	8	7.58	0.01	2113	6	1482	46	26	7.48	71	1506	1500	2029	33	2133	0.50	0.80
2012	4	pH 7.67	8	bottle 4	R1	5700	33.441	8	7.58	0.01	2113	6	1482	46	26	7.48	71	1506	1500	2029	33	2133	0.50	0.80
2012	4	pH 7.67	8	bottle 4	R2	6600	33.441	8	7.58	0.01	2113	6	1482	46	26	7.48	71	1506	1500	2029	33	2133	0.50	0.80
2012	4	pH 7.67	8	bottle 4	R3	3800	33.441	8	7.58	0.01	2113	6	1482	46	26	7.48	71	1506	1500	2029	33	2133	0.50	0.80
2012	4	pH 7.67	8	bottle 5	R1	2800	33.441	8	7.58	0.01	2113	6	1482	46	26	7.48	71	1506	1500	2029	33	2133	0.50	0.80
2012	4	pH 7.67	8	bottle 5	R2	5300	33.441	8	7.58	0.01	2113	6	1482	46	26	7.48	71	1506	1500	2029	33	2133	0.50	0.80
2012	4	pH 7.67	8	bottle 5	R3	3200	33.441	8	7.58	0.01	2113	6	1482	46	26	7.48	71	1506	1500	2029	33	2133	0.50	0.80
2012	2	pH in situ	18	bottle 1	R1	140	33.441	8	8.18	0.01	2328	6	397	10	26	8.08	18	374	372	2004	131	2152	1.98	3.14
2012	2	pH in situ	18	bottle 1	R2	340	33.441	8	8.18	0.01	2328	6	397	10	26	8.08	18	374	372	2004	131	2152	1.98	3.14
2012	2	pH in situ	18	bottle 1	R3	190	33.441	8	8.18	0.01	2328	6	397	10	26	8.08	18	374	372	2004	131	2152	1.98	3.14
2012	2	pH in situ	18	bottle 2	R1	540	33.441	8	8.18	0.01	2328	6	397	10	26	8.08	18	374	372	2004	131	2152	1.98	3.14
2012	2	pH in situ	18	bottle 2	R2	420	33.441	8	8.18	0.01	2328	6	397	10	26	8.08	18	374	372	2004	131	2152	1.98	3.14
2012	2	pH in situ	18	bottle 2	R3	540	33.441	8	8.18	0.01	2328	6	397	10	26	8.08	18	374	372	2004	131	2152	1.98	3.14
2012	2	pH in situ	18	bottle 3	R1	480	33.441	8	8.18	0.01	2328	6	397	10	26	8.08	18	374	372	2004	131	2152	1.98	3.14
2012	2	pH in situ	18	bottle 3	R2	450	33.441	8	8.18	0.01	2328	6	397	10	26	8.08	18	374	372	2004	131	2152	1.98	3.14
2012	2	pH in situ	18	bottle 3	R3	500	33.441	8	8.18	0.01	2328	6	397	10	26	8.08	18	374	372	2004	131	2152	1.98	3.14
2012	2	pH in situ	18	bottle 4	R1	270	33.441	8	8.18	0.01	2328	6	397	10	26	8.08	18	374	372	2004	131	2152	1.98	3.14
2012	2	pH in situ	18	bottle 4	R2	370	33.441	8	8.18	0.01	2328	6	397	10	26	8.08	18	374	372	2004	131	2152	1.98	3.14
2012	2	pH in situ	18	bottle 4	R3	290	33.441	8	8.18	0.01	2328	6	397	10	26	8.08	18	374	372	2004	131	2152	1.98	3.14
2012	2	pH in situ	18	bottle 5	R1	190	33.441	8	8.18	0.01	2328	6	397	10	26	8.08	18	374	372	2004	131	2152	1.98	3.14
2012	2	pH in situ	18	bottle 5	R2	440	33.441	8	8.18	0.01	2328	6	397	10	26	8.08	18	374	372	2004	131	2152	1.98	3.14
2012	2	pH in situ	18	bottle 5	R3	270	33.441	8	8.18	0.01	2328	6	397	10	26	8.08	18	374	372	2004	131	2152	1.98	3.14
2012	2	pH 7.82	18	bottle 1	R1	1660	33.441	8	7.76	0.01	2163	12	1052	24	26	7.66	47	998	994	2036	50	2133	0.77	1.21
2012	2	pH 7.82	18	bottle 1	R2	2010	33.441	8	7.76	0.01	2163	12	1052	24	26	7.66	47	998	994	2036	50	2133	0.77	1.21
2012	2	pH 7.82	18	bottle 1	R3	2200	33.441	8	7.76	0.01	2163	12	1052	24	26	7.66	47	998	994	2036	50	2133	0.77	1.21
2012	2	pH 7.82	18	bottle 2	R1	2600	33.441	8	7.76	0.01	2163	12	1052	24	26	7.66	47	998	994	2036	50	2133	0.77	1.21
2012	2	pH 7.82	18	bottle 2	R2	2370	33.441	8	7.76	0.01	2163	12	1052	24	26	7.66	47	998	994	2036	50	2133	0.77	1.21
2012	2	pH 7.82	18	bottle 2	R3	2640	33.441	8	7.76	0.01	2163	12	1052	24	26	7.66	47	998	994	2036	50	2133	0.77	1.21
2012	2	pH 7.82	18	bottle 3	R1	990	33.441	8	7.76	0.01	2163	12	1052	24	26	7.66	47	998	994	2036	50	2133	0.77	1.21
2012	2	pH 7.82	18	bottle 3	R2	1230	33.441	8	7.76	0.01	2163	12	1052	24	26	7.66	47	998	994	2036	50	2133	0.77	1.21
2012	2	pH 7.82	18	bottle 3	R3	1330	33.441	8	7.76	0.01	2163	12	1052	24	26	7.66	47	998	994	2036	50	2133	0.77	1.21
2012	2	pH 7.82	18	bottle 4	R1	1800	33.441	8	7.76	0.01	2163	12	1052	24	26	7.66	47	998	994	2036	50	2133	0.77	1.21
2012	2	pH 7.82	18	bottle 4	R2	1440	33.441	8	7.76	0.01	2163	12	1052	24	26	7.66	47	998	994	2036	50	2133	0.77	1.21
2012	2	pH 7.82	18	bottle 4	R3	1520	33.441	8	7.76	0.01	2163	12	1052	24	26	7.66	47	998	994	2036	50	2133	0.77	1.21
2012	2	pH 7.82	18	bottle 5	R1	2260	33.441	8	7.76	0.01	2163	12	1052	24	26	7.66	47	998	994	2036	50	2133	0.77	1.21
2012	2	pH 7.82	18	bottle 5	R2	1790	33.441	8	7.76	0.01	2163	12	1052	24	26	7.66	47	998	994	2036	50	2133	0.77	1.21
2012	2	pH 7.82	18	bottle 5	R3	2450	33.441	8	7.76	0.01	2163	12	1052	24	26	7.66	47	998	994	2036	50	2133	0.77	1.21
2012	2	pH 7.67	18	bottle 1	R1	12800	33.441	8	7.62	0.01	2099	12	1442	37	26	7.52	64	1359	1353	2007	36	2108	0.55	0.87
2012	2	pH 7.67	18	bottle 1	R2	13100	33.441	8	7.62	0.01	2099	12	1442	37	26	7.52	64	1359	1353	2007	36	2108	0.55	0.87
2012	2	pH 7.67	18	bottle 1	R3	14200	33.441	8	7.62	0.01	2099	12	1442	37	26	7.52	64	1359	1353	2007	36	2108	0.55	0.87
2012	2	pH 7.67	18	bottle 2	R1	12700	33.441	8	7.62	0.01	2099	12	1442	37	26	7.52	64	1359	1353	2007	36	2108	0.55	0.87
2012	2	pH 7.67	18	bottle 2	R2	11800	33.441	8	7.62	0.01	2099	12	1442	37	26	7.52	64	1359	1353	2007	36	2108	0.55	0.87
2012	2	pH 7.67	18	bottle 2	R3	12000	33.441	8	7.62	0.01	2099	12	1442	37	26	7.52	64	1359	1353	2007	36	2108	0.55	0.87
2012	2	pH 7.67	18	bottle 3	R1	10000	33.441	8	7.62	0.01	2099	12	1442	37	26	7.52	64	1359	1353	2007	36	2108	0.55	0.87
2012	2	pH 7.67	18	bottle 3	R2	5200	33.441	8	7.62	0.01	2099	12	1442	37	26	7.52	64	1359	1353	2007	36	2108	0.55	0.87
2012	2	pH 7.67	18	bottle 3	R3	12900	33.441	8	7.62	0.01	2099	12	1442	37	26	7.52	64	1359	1353	2007	36	2108	0.55	0.87
2012	2	pH 7.67	18	bottle 4	R1	9100	33.441	8	7.62	0.01	2099	12	1442	37	26	7.52	64	1359	1353	2007	36	2108	0.55	0.87
2012	2	pH 7.67	18	bottle 4	R2	9500	33.441	8	7.62	0.01	2099	12	1442	37	26	7.52	64	1359	1353	2007	36	2108	0.55	0.87
2012	2	pH 7.67	18	bottle 4	R3	11700	33.441	8	7.62	0.01	2099	12	1442	37	26	7.52	64	1359	1353	2007	36	2108	0.55	0.87
2012	2	pH 7.67	18	bottle 5	R1	7000	33.441	8	7.62	0.01	2099	12	1442	37	26	7.52	64	1359	1353	2007	36	2108	0.55	0.87
2012	2	pH 7.67	18	bottle 5	R2	5400	33.441	8	7.62	0.01	2099	12	1442	37	26	7.52	64	1359	1353	2007	36	2108	0.55	0.87
2012	2	pH 7.67	18	bottle 5	R3	5800	33.441	8	7.62	0.01	2099	12	1442	37	26	7.52	64	1359	1353	2007	36	2108	0.55	0.87
2012	4	pH in situ	18	bottle 1	R1	170	33.441	8	8.14	0.01	2327	9	406	14	26	8.04	20	415	413	2028	120	2168	1.83	2.90
2012	4	pH in situ	18	bottle 1	R2	160	33.441	8	8.14	0.01	2327	9	406	14	26	8.04	20	415	413	2028	120	2168	1.83	2.90
2012	4	pH in situ	18	bottle 1	R3	170	33.441	8	8.14	0.01	2327	9	406	14	26	8.04	20	415	413	2028	120	2168	1.83	2.90
2012	4	pH in situ	18	bottle 2	R1	120	33.441	8	8.14	0.01	2327	9	406	14	26	8.04	20	415	413	2028	120	2168	1.83	2.90
2012	4	pH in situ	18	bottle 2	R2	200	33.441	8	8.14	0.01	2327	9	406	14	26	8.04	20	415	413	2028	120	2168	1.83	2.90
2012	4	pH in situ	18	bottle 2	R3	200	33.441	8	8.14	0.01	2327	9	406	14	26	8.04	20	415	413	2028	120	2168	1.83	2.90
2012	4	pH in situ	18	bottle 3	R1	320	33.441	8	8.14	0.01	2327	9	406	14	26	8.04	20	415	413	2028	120	2168	1.83	2.90
2012	4	pH in situ	18	bottle 3	R2	180	33.441	8	8.14	0.01	2327	9	406	14	26	8.04	20	415	413	2028	120	2168	1.83	2.90
2012	4	pH in situ	18	bottle 3	R3	190	33.441	8	8.14	0.01	2327	9	406	14	26	8.04	20	415	413	2028	120	2168	1.83	2.90
2012	4	pH in situ	18	bottle 4	R1	290	33.441	8	8.14	0.01	2327	9	406	14	26	8.04	20	415	413	2028	120	2168	1.83	2.90
2012	4	pH in situ	18	bottle 4	R2	170	33.441	8	8.14	0.01	2327	9	406	14	26	8.04	20	415	413	2028	120	2168	1.83	2.90
2012	4	pH in situ	18	bottle 4	R3	110	33.441	8	8.14	0.01	2327	9	406	14	26	8.04	20	415	413	2028	120	2168	1.83	2.90
2012	4	pH in situ	18	bottle 5	R1	100	33.441	8	8.14	0.01	2327	9	406	14	26	8.04	20	415	413	2028	120	2168	1.83	2.90
2012	4	pH in situ	18	bottle 5	R2	90	33.441	8	8.14	0.01	2327	9	406	14	26	8.04	20	415	413	2028	120	2168	1.83	2.90
2012	4	pH in situ	18	bottle 5	R3	150	33.441	8	8.14	0.01	2327	9	406	14	26	8.04	20	415	413	2028	120	2168	1.83	2.90
2012	4	pH 7.82	18	bottle 1	R1	1230	33.441	8	7.70	0.01	2158	8	1139	40	26	7.60	54	1152	1148	2046	44	2145	0.67	1.06
2012	4	pH 7.82	18	bottle 1	R2	1390	33.441	8	7.70	0.01	2158	8	1139	40	26	7.60	54	1152	1148	2046	44	2145	0.67	1.06
2012	4	pH 7.82	18	bottle 1	R3	1550	33.441	8	7.70	0.01	2158	8	1139	40	26	7.60	54	1152	1148	2046	44	2145	0.67	1.06
2012	4	pH 7.82	18	bottle 2	R1	710	33.441	8	7.70	0.01	2158	8	1139	40	26	7.60	54	1152	1148	2046	44	2145	0.67	1.06
2012	4	pH 7.82	18	bottle 2	R2	540	33.441	8	7.70	0.01	2158	8	1139	40	26	7.60	54	1152	1148	2046	44	2145	0.67	1.06
2012	4	pH 7.82	18	bottle 2	R3	260	33.441	8	7.70	0.01	2158	8	1139	40	26	7.60	54	1152	1148	2046	44	2145	0.67	1.06
2012	4	pH 7.82	18	bottle 3	R1	1250	33.441	8	7.70	0.01	2158	8	1139	40	26	7.60	54	1152	1148	2046	44	2145	0.67	1.06
2012	4	pH 7.82	18	bottle 3	R2	970	33.441	8	7.70	0.01	2158	8	1139	40	26	7.60	54	1152	1148	2046	44	2145	0.67	1.06
2012	4	pH 7.82	18	bottle 3	R3	1180	33.441	8	7.70	0.01	2158	8	1139	40	26	7.60	54	1152	1148	2046	44	2145	0.67	1.06
2012	4	pH 7.82	18	bottle 4	R1	1060	33.441	8	7.70	0.01	2158	8	1139	40	26	7.60	54	1152	1148	2046	44	2145	0.67	1.06
2012	4	pH 7.82	18	bottle 4	R2	1190	33.441	8	7.70	0.01	2158	8	1139	40	26	7.60	54	1152	1148	2046	44	2145	0.67	1.06
2012	4	pH 7.82	18	bottle 4	R3	1220	33.441	8	7.70	0.01	2158	8	1139	40	26	7.60	54	1152	1148	2046	44	2145	0.67	1.06
2012	4	pH 7.82	18	bottle 5	R1	810	33.441	8	7.70	0.01	2158	8	1139	40	26	7.60	54	1152	1148	2046	44	2145	0.67	1.06
2012	4	pH 7.82	18	bottle 5	R2	440	33.441	8	7.70	0.01	2158	8	1139	40	26	7.60	54	1152	1148	2046	44	2145	0.67	1.06
2012	4	pH 7.82	18	bottle 5	R3	960	33.441	8	7.70	0.01	2158	8	1139	40	26	7.60	54	1152	1148	2046	44	2145	0.67	1.06
2012	4	pH 7.67	18	bottle 1	R1	6300	33.441	8	7.58	0.01	2113	6	1482	46	26	7.48	71	1506	1500	2029	33	2133	0.50	0.80
2012	4	pH 7.67	18	bottle 1	R2	5900	33.441	8	7.58	0.01	2113	6	1482	46	26	7.48	71	1506	1500	2029	33	2133	0.50	0.80
2012	4	pH 7.67	18	bottle 1	R3	6700	33.441	8	7.58	0.01	2113	6	1482	46	26	7.48	71	1506	1500	2029	33	2133	0.50	0.80
2012	4	pH 7.67	18	bottle 2	R1	8000	33.441	8	7.58	0.01	2113	6	1482	46	26	7.48	71	1506	1500	2029	33	2133	0.50	0.80
2012	4	pH 7.67	18	bottle 2	R2	5400	33.441	8	7.58	0.01	2113	6	1482	46	26	7.48	71	1506	1500	2029	33	2133	0.50	0.80
2012	4	pH 7.67	18	bottle 2	R3	5500	33.441	8	7.58	0.01	2113	6	1482	46	26	7.48	71	1506	1500	2029	33	2133	0.50	0.80
2012	4	pH 7.67	18	bottle 3	R1	4000	33.441	8	7.58	0.01	2113	6	1482	46	26	7.48	71	1506	1500	2029	33	2133	0.50	0.80
2012	4	pH 7.67	18	bottle 3	R2	4500	33.441	8	7.58	0.01	2113	6	1482	46	26	7.48	71	1506	1500	2029	33	2133	0.50	0.80
2012	4	pH 7.67	18	bottle 3	R3	4600	33.441	8	7.58	0.01	2113	6	1482	46	26	7.48	71	1506	1500	2029	33	2133	0.50	0.80
2012	4	pH 7.67	18	bottle 4	R1	5100	33.441	8	7.58	0.01	2113	6	1482	46	26	7.48	71	1506	1500	2029	33	2133	0.50	0.80
2012	4	pH 7.67	18	bottle 4	R2	4500	33.441	8	7.58	0.01	2113	6	1482	46	26	7.48	71	1506	1500	2029	33	2133	0.50	0.80
2012	4	pH 7.67	18	bottle 4	R3	5000	33.441	8	7.58	0.01	2113	6	1482	46	26	7.48	71	1506	1500	2029	33	2133	0.50	0.80
2012	4	pH 7.67	18	bottle 5	R1	4500	33.441	8	7.58	0.01	2113	6	1482	46	26	7.48	71	1506	1500	2029	33	2133	0.50	0.80
2012	4	pH 7.67	18	bottle 5	R2	3500	33.441	8	7.58	0.01	2113	6	1482	46	26	7.48	71	1506	1500	2029	33	2133	0.50	0.80
2012	4	pH 7.67	18	bottle 5	R3	4300	33.441	8	7.58	0.01	2113	6	1482	46	26	7.48	71	1506	1500	2029	33	2133	0.50	0.80