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Seasonally chemical weathering and CO2 consumption flux of Lake Qinghai river system in the northeastern Tibetan Plateau

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Abstract

The major cation and anion compositions of waters from the Lake Qinghai river system (LQRS) in the northeastern Tibetan Plateau were measured. The waters were collected seasonally from five main rivers during pre-monsoon (late May), monsoon (late July), and post-monsoon (middle October). The LQRS waters are all very alkaline and have high concentrations of TDS (total dissolved solids) compared to rivers draining the Himalayas and the southeastern Tibetan Plateau. Seasonal variations in the water chemistry show that, except the Daotang River, the TDS concentration is high in October and low in July in the LQRS waters. The forward models were used to quantify the input of three main rivers (Buha River, Shaliu River, and Hargai River) from rain, halite, carbonates, and silicates. The results suggest that (1) atmospheric input is the first important source for the waters of the Buha River and the Shaliu River, contributing 36–57% of the total dissolved cations, (2) carbonate weathering input and atmospheric input have equal contribution to the Hargai River water, (3) carbonate weathering has higher contribution to these rivers than silicate weathering, and (4) halite is also important source for the Buha River. The Daotang River water is dominated by halite input owing to its underlying old lacustrine sediments. The water compositions of the Heima River are controlled by carbonate weathering and rainfall input in monsoon season, and groundwater input may be important in pre-monsoon and post-monsoon seasons. After being corrected the atmospheric input, average CO2 drawdown via silicate weathering in the LQRS is 35 × 103 mol/km2 per year, with highest in monsoon season, lower than Himalayas and periphery of Tibetan Plateau rivers but higher than some rivers draining shields.

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References

  • Berner EK, Berner RA (1996) Global environment: water, air, and geochemical cycles. Prentice–Hall, Englewood Cliffs

    Google Scholar 

  • Berner RA, Lasaga AC, Garrels RM (1983) The carbonate–silicate geochemical cycle and its effect on atmospheric carbon dioxide over the past 100 million years. Am J Sci 283:641–683

    Google Scholar 

  • Bethke CM (2002) The geochemist’s workbench 4.0. p 224

  • Bickle MJ, Chapman HJ, Bunbury J, Harris NBW, Fairchild IJ, Ahmad T, Pomiès C (2005) Relative contributions of silicate and carbonate rocks to riverine Sr fluxes in the headwaters of the Ganges. Geochim Cosmochim Acta 69:2221–2240

    Article  Google Scholar 

  • Dalai TK, Krishnaswami S, Sarin MM (2002) Major ion chemistry in the headwaters of the Yamuna river system: chemical weathering, its temperature dependence and CO2 consumption in the Himalaya. Geochim Cosmochim Acta 66:3397–3416

    Article  Google Scholar 

  • Dalai TK, Krishnaswami S, Kumar A (2003) Sr and 87Sr/86Sr in the Yamuna River System in the Himalaya: sources, fluxes, and controls on Sr isotope composition. Geochim Cosmochim Acta 67:2931–2948

    Article  Google Scholar 

  • Das A, Krishnaswami S, Sarin MM, Pande K (2005) Chemical weathering in the Krishna Basin and Western Ghats of the Deccan traps, India: rates of basalt weathering and their controls. Geochim Cosmochim Acta 69:2067–2084

    Article  Google Scholar 

  • Dessert C, Dupré B, Francois LM, Schott J, Gaillardet J, Chakrapani G, Bajpai S (2001) Erosion of Deccan Traps determined by river geochemistry: impact on the global climate and the 87Sr/86Sr ratio of seawater. Earth Planet Sci Lett 188:459–474

    Article  Google Scholar 

  • Ding Y, Liu F (1993) Estimating on water balance elements in the drainage basin of Qinghai Lake. Arid Zone Res 16:25–30

    Google Scholar 

  • Dupré B, Gaillardet J, Rousseau D, Allègre CJ (1996) Major and trace element of river-borne material: the Congo Basin. Geochim Cosmochim Acta 60:1301–1321

    Article  Google Scholar 

  • Edmond JM, Palmer MR, Measures CI, Grant B, Stallard RF (1995) The fluvial geochemistry and denudation rate of the Guayana Shield in Venezuela, Colombia and Brazil. Geochim Cosmochim Acta 59:3301–3325

    Article  Google Scholar 

  • English N, Quade J, DeCelles P, Garzione C (2000) Geologic control of Sr and major element chemistry in Himalayan Rivers, Nepal. Geochim Cosmochim Acta 64:2549–2566

    Article  Google Scholar 

  • Gaillardet J, Dupré B, Allègre CJ, Négrel P (1997) Chemical and physical denudation in the Amazon River Basin. Chem Geol 142:141–173

    Article  Google Scholar 

  • Gaillardet J, Dupré B, Louvat P, Allègre CJ (1999) Global silicate weathering and CO2 consumption rates deduced from the chemistry of large rivers. Chem Geol 159:3–30

    Article  Google Scholar 

  • Galy A, France-Lanord C (1999) Weathering processes in the Ganges–Brahmaputra basin and the riverine alkalinity budget. Chem Geol 159:31–60

    Article  Google Scholar 

  • Galy A, France-Lanord C (2001) Higher erosion rates in the Himalaya: geochemical constrains on riverine fluxes. Geology 29:23–26

    Article  Google Scholar 

  • Gordeev VV, Sidorov IS (1993) Concentrations of major elements and their outflow into the Laptev Sea by the Lena river. Mar Chem 43:34–45

    Article  Google Scholar 

  • Grosbois C, Négrel P, Fouillac C, Grimaud D (2000) Chemical and isotopic characterization of the dissolved load of the Loire River. Chem Geol 170:179–201

    Article  Google Scholar 

  • Hasnain SI, Thayyen RJ (1999) Controls on the major–ion chemistry of the Dokriani glacier meltwaters, Ganga Basin, Garhwal Himalaya, India. J Glaciol 45:87–92

    Google Scholar 

  • Hren MT, Chamberlain CP, Hilley GE, Blisniuk PM, Bookhagen B (2007) Major ion chemistry of the Yarlung Tsangpo–Brahmaputra river: Chemical weathering, erosion, and CO2 consumption in the southern Tibetan plateau and eastern syntaxis of the Himalaya. Geochim Cosmochim Acta 71:2907–2935

    Article  Google Scholar 

  • Hu MH, Stallard RF, Edmond JM (1982) Major ion chemistry of some large Chinese rivers. Nature 298:550–553

    Article  Google Scholar 

  • Huh Y, Edmond JM (1999) The fluvial geochemistry of the rivers of Eastern Siberia: III. Tributaries of the Lena and Anabar draining the basement terrain of the Siberian Craton and the Trans-Baikal Highlands. Geochim Cosmochim Acta 63(7–8):967–987

    Article  Google Scholar 

  • Huh Y, Tsoi MY, Zaitsev A, Edmond JM (1998) The fluvial geochemistry of the rivers of Eastern Siberia: I. Tributaries of the Lena River draining the sedimentary platform of the Siberian Craton. Geochim Cosmochim Acta 62:1657–1676

    Article  Google Scholar 

  • Jacobson AD, Blum JD, Walter LM (2002) Reconciling the elemental and Sr isotope composition of Himalayan weathering fluxes: insights from the carbonate geochemistry of stream waters. Geochim Cosmochim Acta 66:3417–3429

    Article  Google Scholar 

  • Jin ZD, Cao J, Wu J, Wang S (2006a) A Rb/Sr record of catchment weathering response to Holocene climate change in Inner Mongolia. Earth Surf Process Landform 31:285–291

    Article  Google Scholar 

  • Jin ZD, Li FC, Cao JJ, Wang SM, Yu JM (2006b) Geochemistry of Daihai Lake sediments, Inner Mongolia, north China: implications for provenance, sedimentary sorting, and catchment weathering. Geomorphology 80:147–163

    Article  Google Scholar 

  • Kang S, Cong Z (2006) Progress in study on precipitation and aerosol chemistry in the Tibetan Plateau. J Glaciol Geocryol 28:371–379

    Google Scholar 

  • Karim A, Veizer J (2000) Weathering processes in the Indus River Basin: implications from riverine carbon, sulfur, oxygen, and strontium isotopes. Chem Geol 170:153–177

    Article  Google Scholar 

  • Krishnaswami S, Singh SK, Dalai TK (1999) Silicate weathering in the Himalaya: role in contributing to major ions and radiogenic Sr to the Bay of Bengal. In: Somayajulu BLK (ed) Ocean science, trends and future directions. Indian National Science Academy and Akademia International, New Delhi, pp 23–51

    Google Scholar 

  • Lal D, Harris NBW, Sharma KK, Gu Z, Ding L, Liu T, Dong W, Caffee MW, Jull AJT (2003) Erosion history of the Tibetan Plateau since the last interglacial: constraints from the first studies of cosmogenic 10Be from Tibetan bedrock. Earth Planet Sci Lett 217:33–42

    Article  Google Scholar 

  • Li XY, Xu H, Sun YL, Zhang DS, Yang Z (2007) Lake-level change and water balance analysis at lake Qinghai, west China during recent decades. Water Resour Manag 21:1505–1516

    Article  Google Scholar 

  • LIGCAS (Lanzhou Institute of Geology of Chinese Academy of Sciences) (1979) A synthetical investigation report on Qinghai Lake. Science Press, Beijing, pp 1–23 (in Chinese)

    Google Scholar 

  • LZBCAS (Lanzhou Branch of Chinese Academy of Sciences) (1994) Evolution of recent environment in Qinghai Lake and its prediction. West Center of Resource and Environment. Chinese Academy of Sciences, Science Press, Beijing (in Chinese)

    Google Scholar 

  • Meybeck M (1979) Concentrations des eaux fluviales en éléments majeurs et apports en solution aux océans, Rev. Geol Dyn Geog Phy 21(3):215–246

    Google Scholar 

  • Meybeck M (1981) Pathways of major elements from land to ocean through rivers. In: Martin JM, Burton JD, Eisma D (eds) River inputs to ocean systems. UNEP/IOC/SCOR/UNESCO, Switzerland, pp 18–30

    Google Scholar 

  • Meybeck M (1983) Atmospheric inputs and river transport of dissolved substances. In: Dissolved loads of rivers and surface quality/quantity relationships, vol 141. IAHS Publ, pp 173–192

  • Meybeck M (2003) Global occurrence of major elements in rivers. In: Drever JI (ed) Treatise on geochemistry, surface and ground water, weathering, and soils. Elsevier, Amsterdam, pp 207–223

  • Millot R, Gaillardet J, Dupré B, Allègre CJ (2002) The global control of silicate weathering rates and the coupling with physical erosion: New insights from rivers of the Canadian Shield. Earth Planet Sci Lett 196:83–98

    Article  Google Scholar 

  • Millot R, Gaillardet J, Dupré B, Allègre CJ (2003) Northern latitude chemical weathering rates: clues from the Mackenzie River Basin, Canada. Geochim Cosmochim Acta 67(7):1305–1329

    Article  Google Scholar 

  • Moon S, Huh Y, Qin J, Pho NV (2007) Chemical weathering in the Hong (Red) River basin: Rates of silicate weathering and their controlling factors. Geochim Cosmochim Acta 71(6):1411–1430

    Article  Google Scholar 

  • Négrel P, Allègre CJ, Dupré B, Lewin E (1993) Erosion sources determined by inversion of major and trace element ratios and strontium isotopic ratios in river water: the Congo Basin case. Earth Planet Sci Lett 120:59–76

    Article  Google Scholar 

  • Nijampurkar VN, Sarin MM, Rao DK (1993) Chemical composition of snow and ice from Chota Shigri glacier, Central Himalaya. J Hydrol 151:19–34

    Article  Google Scholar 

  • Pandey SK, Singh AK, Hasnain SI (2001) Hydrochemical characteristics of meltwater draining from Pindari glacier, Kumaon Himalaya. J Geol Soc India 57:519–527

    Google Scholar 

  • Probst JL, Nkounkou RR, Krempp G, Bricquet JP, Thiebaux JP, Olivry JC (1992) Dissolved major elements exported by the Congo and the Ubangui rivers during the period 1987–1989. J Hydrol 135:237–257

    Article  Google Scholar 

  • Qin J, Huh Y, Edmond JM, Du G, Ran J (2006) Chemical and physical weathering in the Min Jiang, a headwater tributary of the Yangtze River. Chem Geol 227(1–2):53–69

    Article  Google Scholar 

  • Raymo ME, Ruddiman WF (1992) Tectonic forcing of late Cenozoic climate. Nature 359:117–122

    Article  Google Scholar 

  • Sarin MM, Krishnaswami S, Dilli K, Somayajulu BLK, Moore WS (1989) Major ion chemistry of the Ganga–Brahmaputra river system: weathering processes and fluxes to the Bay of Bengal. Geochim Cosmochim Acta 53:997–1009

    Article  Google Scholar 

  • Stallard RF, Edmond JM (1981) Geochemistry of the Amazon 1. Precipitation chemistry and the marine contribution to the dissolved load at the time of peak discharge. J Geophys Res 86:9844–9858

    Article  Google Scholar 

  • Stallard RF, Edmond JM (1983) Geochemistry of the Amazon 2. The influence of geology and weathering environment on the dissolved load. J Geophys Res 88:9671–9688

    Article  Google Scholar 

  • Stallard RF, Edmond JM (1987) Geochemistry of the Amazon 3. Weathering chemistry and limits to dissolved inputs. J Geophys Res 92(C8):8293–8302

    Article  Google Scholar 

  • Sun Y, Li X, Xu H (2007) Daily precipitation and temperature variations in Qinghai Lake watershed in recent 40 years. Arid Meteorol 25(1):7–13

    Google Scholar 

  • Tang J, Xue H, Yu X (2000) The preliminary study on chemical characteristics of precipitation at Mt Waliguan. Acta Sci Circumst 20(4):420–425

    Google Scholar 

  • Velbel M (1993) Temperature dependence of silicate weathering in nature: how strong a negative feedback on long term accumulation of atmospheric CO2 and global greenhouse warming? Geology 21:1059–1062

    Article  Google Scholar 

  • Wake CP, Mayewski PA, Spencer MJ (1990) A review of central Asian glaciochemical data. Ann Glaciol 14:301–306

    Google Scholar 

  • Wake CP, Mayewski PA, Xie Z, Ping W, Li Z (1993) Regional distribution of monsoon and desert dust signals recorded in Asian glaciers. Geophys Res Lett 30:1411–1414

    Article  Google Scholar 

  • Wake CP, Mayewski PA, Li Z, Han J, Qin D (1994a) Modern eolian dust deposition in central Asia. Tellus 46B:220–233

    Google Scholar 

  • Wake CP, Dibb JE, Mayewski PA, Xie Z, Li Z, Ping W, Qin D (1994b) The chemical composition of aerosols over the eastern Himalaya and Tibetan Plateau during low dust periods. Atmos Environ 28A:695–704

    Article  Google Scholar 

  • Wang YQ, Zhang XY, Arimoto R, Cao JJ, Shen ZX (2005) Characteristics of carbonate content and carbon and oxygen isotopic composition of northern China soil and dust aerosol and its application to tracing dust sources. Atmos Environ 39:2631–2642

    Article  Google Scholar 

  • West AJ, Galy A, Bickle MJ (2005) Tectonic and climatic controls on silicate weathering. Earth Planet Sci Lett 235(1–2):211–228

    Article  Google Scholar 

  • White AF, Blum AE (1995) Effects of climate on chemical weathering in watersheds. Geochim Cosmochim Acta 59(9):1729–1747

    Article  Google Scholar 

  • White AF, Blum AE, Schultz MS, Vivit DV, Stonestrom DA, Larson M, Murphy SF, Eberl D (1998) Chemical weathering in a tropical watershed, Luquillo Mountains, Puerto Rico: I. Long-term versus short term weathering fluxes. Geochim Cosmochim Acta 62:209–226

    Article  Google Scholar 

  • Wu L, Huh Y, Qin J, Du G, van Der Lee S (2005) Chemical weathering in the Upper Huang He (Yellow River) draining the eastern Tibetan Plateau. Geochim Cosmochim Acta 69(22):5279–5294

    Article  Google Scholar 

  • Wu WH, Xu SJ, Yang JD, Yin HW (2008) Silicate weathering and CO2 consumption deduced from the seven Chinese rivers originating in the Qinghai-Tibet Plateau. Chem Geol 249:307–320

    Article  Google Scholar 

  • Zhang X (2001) Source distributions, emission, transport, deposition of Asian dust and loess accumulation. Quat Sci 21:29–40

    Google Scholar 

  • Zhang DD, Jim CY, Peart MR (2003a) Rapid changes of precipitation pH in Qinghai Province, the northeastern Tibetan Plateau. Sci Total Environ 305:241–248

    Article  Google Scholar 

  • Zhang DD, Peart M, Jim CY, He YQ, Li BS, Chen JAA (2003b) Precipitation chemistry of Lhasa and other remote towns, Tibet. Atmos Environ 37:231–240

    Article  Google Scholar 

  • Zhang D, Shi C, Jia L (2004) A study of chemical properties of rains on the Tibetan Plateau. Acta Sci Circumst 24(3):555–557

    Google Scholar 

  • Zhang D, Shi C, Jia L (2005) Analysis on chemical composition of rainfall on the Tibet Plateau. Arid Zone Res 22(4):471–475

    Google Scholar 

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Acknowledgments

This work has been financially supported by National Natural Science Foundation of China through grants 40599423 and 40873082, and by National Basic Research Program of China (2004CB720200). We especially thank Associate Professor Zhu Yuxin in Nanjing Institute of Geography and Limnology, Chinese Academy of Sciences, Miss Sun Yufang in Nanjing Institute of Soil Sciences, Chinese Academy of Sciences, and Miss Zhang Ting in Institute of Earth Environment, Chinese Academy of Sciences, for their kind help and suggestions to sample analyses and laboratory work. Thanks are extended to Professor Yang Bo in Qinghai Institute of Salt Lake, Chinese Academy of Sciences for his assistance with sample collection.

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Zhang, F., Jin, Z., Hu, G. et al. Seasonally chemical weathering and CO2 consumption flux of Lake Qinghai river system in the northeastern Tibetan Plateau. Environ Earth Sci 59, 297–313 (2009). https://doi.org/10.1007/s12665-009-0027-3

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